The surface Fermi arc, as a hallmark of Weyl semimetals (WSMs), has been well known in current research, but it remains a challenge to unveil novel phenomena associated with the Fermi arc. Here, we predict a heretofore unrecognized process in WSMs, namely, the photoinduced transition between the bulk states and the Fermi arc. We find this process is significant and can lead to a large effective three-dimensional shift current on the boundaries with the Fermi arc in wide terahertz range. Moreover, due to the low symmetry of the boundaries, the surface photogalvanic effect predicted here can appear in a large class of WSMs that do not have bulk shift current. Hence, our work not only unveils a hidden photogalvanic effect in WSMs but also suggests that all the WSMs are promising material candidates for developing efficient terahertz photodetectors.
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