Magnetic anisotropy and critical behavior of the quaternary van der Waals ferromagnetic material $bf CrGe_{delta}Si_{1-delta}Te_3$


الملخص بالإنكليزية

Recently, two-dimensional ferromagnetism in the family of Chromium compounds $rm CrXTe_3 (X=Si, Ge)$ has attracted a broad research interest. Despite the structural similarity in $rm CrTe_6$ octahedra, the size effect of inserted Ge or Si dimer contributes to significant differences in magnetism. Here, we report a new quaternary van der Waals ferromagnetic material $rm CrGe_{delta}Si_{1-delta}Te_3$ synthesized by flux method. Ge substitution in Si site results in the lattice expansion, further increasing the Curie temperature and reducing the magnetic anisotropy. The critical behavior of $rm Cr_{0.96}Ge_{0.17}Si_{0.82}Te_3$ has been studied by specific heat as well as magnetization measurements. And the extracted critical exponents are self-consistent and well-obeying the scaling laws, which are closer to the 2D Ising model with interaction decaying as $J(r)approx r^{-3.44}$.

تحميل البحث