Using the concept of non-degenerate Bell inequality, we show that quantum entanglement, the critical resource for various quantum information processing tasks, can be quantified for any unknown quantum states in a semi-device-independent manner, where the quantification is based on the experimentally obtained probability distribution and beforehand knowledge on quantum dimension only. Specifically, as an application of our approach on multi-level systems, we experimentally quantify the entanglement of formation and the entanglement of distillation for qutrit-qutrit quantum systems. In addition, to demonstrate our approach for multi-partite systems, we further quantify the geometry measure of entanglement of three-qubit quantum systems. Our results supply a general way to reliably quantify entanglement in multi-level and multi-partite systems, thus paving the way to characterize many-body quantum systems by quantifying involved entanglement.
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