The critical nature of the Ni spin state in doped NdNiO$_2$


الملخص بالإنكليزية

Superconductivity with $T_c approx 15K$ was recently found in doped NdNiO$_2$. The Ni$^{1+}$O$_2$ layers are expected to be Mott insulators so hole doping should produce Ni$^{2+}$ with $S=1$, incompatible with robust superconductivity. We show that the NiO$_2$ layers fall inside a ``critical region where the large $pd$ hybridization favors a singlet $^1!A_1$ hole-doped state like in CuO$_2$. However, we find that the superexchange is about one order smaller than in cuprates, thus a magnon ``glue is very unlikely and another mechanism needs to be found.

تحميل البحث