We report the results from a new, highly sensitive ($Delta T_{mb} sim 3 $mK) survey for thermal OH emission at 1665 and 1667 MHz over a dense, 9 x 9-pixel grid covering a $1deg$ x $1deg$ patch of sky in the direction of $l = 105deg, b = +2.50deg$ towards the Perseus spiral arm of our Galaxy. We compare our Green Bank Telescope (GBT) 1667 MHz OH results with archival CO J=1-0 observations from the Five College Radio Astronomy Observatory (FCRAO) Outer Galaxy Survey within the velocity range of the Perseus Arm at these galactic coordinates. Out of the 81 statistically-independent pointings in our survey area, 86% show detectable OH emission at 1667 MHz, and 19% of them show detectable CO emission. We explore the possible physical conditions of the observed features using a set of diffuse molecular cloud models. In the context of these models, both OH and CO disappear at current sensitivity limits below an A$_{rm v}$ of 0.2, but the CO emission does not appear until the volume density exceeds 100-200 cm$^{-3}$. These results demonstrate that a combination of low column density A$_{rm v}$ and low volume density $n_{H}$ can explain the lack of CO emission along sight lines exhibiting OH emission. The 18-cm OH main lines, with their low critical density of $n^{*}$ $ sim 1 $ cm$^{-3}$, are collisionally excited over a large fraction of the quiescent galactic environment and, for observations of sufficient sensitivity, provide an optically-thin radio tracer for diffuse H$_2$.
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