We study spectral features of ion velocity and magnetic field correlations in the solar wind and in the magnetosheath using data from the Magnetospheric Multi-Scale (MMS) spacecraft. High resolution MMS observations enable the study of transition of these correlations between their magnetofluid character at larger scales into the sub-proton kinetic range, previously unstudied in spacecraft data. Cross-helicity, angular alignment and energy partitioning is examined over a suit- able range of scales, employing measurements based on the Taylor frozen-in approximation as well as direct two-spacecraft correlation measurements. The results demonstrate signatures of alignment at large scales. As kinetic scales are approached, the alignment between v and b is destroyed by demagnetization of protons.