Type Ia supernovae (SNe Ia) often show high-velocity absorption features (HVFs) in their early phase spectra; however the origin of the HVFs is unknown. We show that a near-Chandrasekhar-mass white dwarf (WD) develops a silicon-rich layer on a carbon-oxygen (CO) core before it explodes as an SN Ia. We calculated the nuclear yields in successive helium shell flashes for 1.0 $M_odot$, 1.2 $M_odot$, and 1.35 $M_odot$ CO WDs accreting helium-rich matter with several mass-accretion rates ranging from $1 times 10^{-7}~M_odot$ yr$^{-1}$ to $7.5 times 10^{-7}~M_odot$ yr$^{-1}$. For the $1.35~M_odot$ WD with the accretion rate of $1.6 times 10^{-7}~M_odot$ yr$^{-1}$, the surface layer developed as helium burning ash and consisted of 40% $^{24}$Mg, 33% $^{12}$C, 23% $^{28}$Si, and a few percent of $^{20}$Ne by weight. For a higher mass accretion rate of $7.5 times 10^{-7}~M_odot$ yr$^{-1}$, the surface layer consisted of 58% $^{12}$C, 31% $^{24}$Mg, and 0.43% $^{28}$Si. For the $1.2~M_odot$ WDs, silicon is produced only for lower mass accretion rates (2% for $1.6 times 10^{-7}~M_odot$ yr$^{-1}$). No substantial silicon ($< 0.07%$) is produced on the $1.0~M_odot$ WD independently of the mass-accretion rate. If the silicon-rich surface layer is the origin of Si II HVFs, its characteristics are consistent with that of mass increasing WDs. We also discuss possible Ca production on very massive WDs ($ gtrsim 1.38~M_odot$).
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