(Abr.) Laser guide stars employed at astronomical observatories provide artificial wavefront reference sources to help correct (in part) the impact of atmospheric turbulence on astrophysical observations. Following the recent commissioning of the 4 Laser Guide Star Facility (4LGSF) on UT4 at the VLT, we characterize the spectral signature of the uplink beams from the 22W lasers to assess the impact of laser scattering from the 4LGSF on science observations. We use the MUSE optical integral field spectrograph to acquire spectra at a resolution of R~3000 of the uplink laser beams over the wavelength range of 4750AA to 9350AA. We report the first detection of laser-induced Raman scattering by N2, O2, CO2, H2O and (tentatively) CH4 molecules in the atmosphere above the astronomical observatory of Cerro Paranal. In particular, our observations reveal the characteristic spectral signature of laser photons -- but 480AA to 2210AA redder than the original laser wavelength of 5889.959AA -- landing on the 8.2m primary mirror of UT4 after being Raman-scattered on their way up to the sodium layer. Laser-induced Raman scattering is not unique to the observatory of Cerro Paranal, but common to any astronomical telescope employing a laser-guide-star (LGS) system. It is thus essential for any optical spectrograph coupled to a LGS system to handle thoroughly the possibility of a Raman spectral contamination via a proper baffling of the instrument and suitable calibrations procedures. These considerations are particularly applicable for the HARMONI optical spectrograph on the upcoming Extremely Large Telescope. At sites hosting multiple telescopes, laser collision prediction tools also ought to account for the presence of Raman emission from the uplink laser beam(s) to avoid the unintentional contamination of observations acquired with telescopes in the vicinity of a LGS system.
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