A new magnetic phase in the nickelate perovskite TlNiO$_3$


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The RNiO$_3$ perovskites are known to order antiferromagnetically below a material-dependent Neel temperature $T_text{N}$. We report experimental evidence indicating the existence of a second magnetically-ordered phase in TlNiO$_3$ above $T_text{N} = 104$ K, obtained using nuclear magnetic resonance and muon spin rotation spectroscopy. The new phase, which persists up to a temperature $T_text{N}^* = 202$ K, is suppressed by the application of an external magnetic field of approximately 1 T. It is not yet known if such a phase also exists in other perovskite nickelates.

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