Using a kilojoule class laser, we demonstrate for the first time that high-contrast picosecond pulses are advantageous for ion acceleration. We show that a laser pulse with optimum duration and a large focal spot accelerates electrons beyond the ponderomotive energy. This anomalous electron heating enables efficient ion acceleration reaching 52 MeV at an intensity of 1.2X10^19 Wcm^-2. The proton energy observed agrees quantitatively with a one-dimensional plasma expansion model newly developed by taking the anomalous heating effect into account. The heating process is confirmed by both measurements with an electron spectrometer and a one-dimensional particle-in-cell simulation. By extending the pulse duration to 6 ps, 5% energy conversion efficiency to protons (50 J out of 1 kJ laser energy) is achieved with an intensity of 10^18-Wcm^-2. The present results are quite encouraging for realizing ion-driven fast ignition and novel ion beamlines.
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