We investigate several aspects of realizing quantum computation using entangled polar molecules in pendular states. Quantum algorithms typically start from a product state |00...0> and we show that up to a negligible error, the ground states of polar molecule arrays can be considered as the unentangled qubit basis state |00...0>. This state can be prepared by simply allowing the system to reach thermal equilibrium at low temperature (<1 mK). We also evaluate entanglement, characterized by the concurrence of pendular state qubits in dipole arrays as governed by the external electric field, dipole-dipole coupling and number N of molecules in the array. In the parameter regime that we consider for quantum computing, we find that qubit entanglement is modest, typically no greater than 0.0001, confirming the negligible entanglement in the ground state. We discuss methods for realizing quantum computation in the gate model, measurement based model, instantaneous quantum polynomial time circuits and the adiabatic model using polar molecules in pendular states.
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