Dust properties appear to vary according to the environment in which the dust evolves. Previous observational indications of these variations in the FIR and submm spectral range are scarce and limited to specific regions of the sky. To determine whether these results can be generalised to larger scales, we study the evolution in dust emissivities from the FIR to mm wavelengths, in the atomic and molecular ISM, along the Galactic plane towards the outer Galaxy. We correlate the dust FIR to mm emission with the HI and CO emission. The study is carried out using the DIRBE data from 100 to 240 mic, the Archeops data from 550 mic to 2.1 mm, and the WMAP data at 3.2 mm (W band), in regions with Galactic latitude |b| < 30 deg, over the Galactic longitude range (75 deg < l < 198 deg) observed with Archeops. In all regions studied, the emissivity spectra in both the atomic and molecular phases are steeper in the FIR (beta = 2.4) than in the submm and mm (beta = 1.5). We find significant variations in the spectral shape of the dust emissivity as a function of the dust temperature in the molecular phase. Regions of similar dust temperature in the molecular and atomic gas exhibit similar emissivity spectra. Regions where the dust is significantly colder in the molecular phase show a significant increase in emissivity for the range 100 - 550 mic. This result supports the hypothesis of grain coagulation in these regions, confirming results obtained over small fractions of the sky in previous studies and allowing us to expand these results to the cold molecular environments in general of the outer MW. We note that it is the first time that these effects have been demonstrated by direct measurement of the emissivity, while previous studies were based only on thermal arguments.
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