The electronic Raman scattering in overdoped (Y,Ca)Ba2Cu3Oy was investigated with changing hole concentration in the superconducting state. It was found that the superconducting responses such as the pair-breaking peaks in the A1g and B1g spectra and the anisotropy of the pair-breaking peak in XX and YY polarizations radically change at around the carrier doping p=0.19. Since both a- and c-axis resistivities strongly suggest the closing of pseudogap at p~0.18, the observed change at p=0.19 in superconducting Raman response is attributed to the electronic crossover due to the collapse of the pseudogap.
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