Thermal Canting of Spin-Bond Order


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Magnetism arising from coupled spin and spatial degrees of freedom underlies the properties of a broad array of physical systems. We study here the interplay between correlations in spin and space for the quantum compass model in a finite external field, using quantum Monte Carlo methods. We find that finite temperatures cant the spin and space (bond) correlations, with increasing temperature even reorienting spin correlations between orthogonal spatial directions. We develop a coupled mean field theory to understand this effect in terms of the underlying quantum critical properties of crossed Ising chains in transverse fields and an effective field that weakens upon increasing temperature. Thermal canting offers an experimental signature of spin-bond anisotropy.

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