اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدIntrinsic Localized Modes Observed in the High Temperature Vibrational Spectrum of NaI
133
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
Inelastic neutron measurements of the high-temperature lattice excitations in NaI show that in thermal equilibrium at 555 K an intrinsic mode, localized in three dimensions, occurs at a single frequency near the center of the spectral phonon gap, polarized along [111]. At higher temperatures the intrinsic localized mode gains intensity. Higher energy inelastic neutron and x-ray scattering measurements on a room-temperature NaI crystal indicate that the creation energy of the ground state of the intrinsic localized mode is 299 meV.
قيم البحث
اقرأ أيضاً
The possibility of thermal excitation of intrinsic localized modes (ILMs) arising from anharmonicity in ionic perfect crystals is studied numerically for realistic model systems in one and three dimensions. Implications are discussed for an interesti
ng high-temperature feature seen in earlier inelastic neutron scattering experiments on single crystal NaI. The general conclusion is that ILM formation energies are far too large for thermal excitation of ILMs to account for the observed feature in a pure crystal.
A microscopic theory for electronic spectrum of the CuO2 plane within an effective p-d Hubbard model is proposed. Dyson equation for the single-electron Green function in terms of the Hubbard operators is derived which is solved self-consistently for
the self-energy evaluated in the noncrossing approximation. Electron scattering on spin fluctuations induced by kinematic interaction is described by a dynamical spin susceptibility with a continuous spectrum. Doping and temperature dependence of electron dispersions, spectral functions, the Fermi surface and the coupling constant are studied in the hole doped case. At low doping, an arc-type Fermi surface and a pseudogap in the spectral function are observed.
We study a nonuniversal contribution to the dephasing rate of conduction electrons due to local vibrational modes. The inelastic scattering rate is strongly influenced by multiphonon excitations, exhibiting oscillatory behaviour. For higher frequenci
es, it saturates to a finite, coupling dependent value. In the strong coupling limit, the phonon is almost completely softened, and the inelastic cross section reaches its maximal value. This represents a magnetic field insensitive contribution to the dephasing time in mesoscopic systems, in addition to magnetic impurities.
The spectrum of the strongly correlated systems usually shows resonant peaks at finite energy, with examples in the 115 Ce family which are reproduced by the dynamical mean-field theory. A similar structure has been seen recently in the orbitally sel
ective Mott (OSM) phase of two-band model, known as doublon-holon bound state, with implications on the fate of such phase in the zero Hunds coupling limit. We show that these features can be captured with the slave-particle methods once their Hilbert space is taken into account. We use slave-spin calculations, justifiable in the limit of large dimensions, to explicitly demonstrate this and compare the results with dynamical mean-field theory.
We study a disordered vibrational model system, where the spring constants k are chosen from a distribution P(k) ~ 1/k above a cut-off value k_min > 0. We can motivate this distribution by the presence of free volume in glassy materials. We show that
the model system reproduces several important features of the boson peak in real glasses: (i) a low-frequency excess contribution to the Debye density of states, (ii) the hump of the specific heat c_V(T) including the power-law relation between height and position of the hump, and (iii) the transition to localized modes well above the boson peak frequency.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
