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We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while decoupling from the noisy spin-bath, which otherwise limits the detection sensitivity. As a proof-of-principle we: (I) observe coherent oscillations between the NV center and a weakly coupled nuclear spin, (II) demonstrate nuclear bath cooling which prolongs the coherence time of the NV sensor by more than a factor of five. Our results provide a route to nanometer scale magnetic resonance imaging, and novel quantum information processing protocols.
Electron spin resonance (ESR) is a useful tool to investigate properties of materials in magnetic fields where high spin polarization of target electron spins is required in order to obtain high sensitivity. However, the smaller magnetic fields becom
Electron and nuclear spins associated with point defects in insulators are promising systems for solid state quantum technology. While the electron spin usually is used for readout and addressing, nuclear spins are exquisite quantum bits and memory s
We report electron spin resonance spectroscopy measurements performed at millikelvin temperatures in a custom-built spectrometer comprising a superconducting micro-resonator at $7$ GHz and a Josephson parametric amplifier. Owing to the small ${sim}10
Quantum emitters respond to resonant illumination by radiating electromagnetic fields. A component of these fields is phase-coherent with the driving tone, while another one is incoherent, consisting of spontaneously emitted photons and forming the f
Hybrid qubit systems combining electronic spins with nearby (proximate) nuclear spin registers offer a promising avenue towards quantum information processing, with even multi-spin error correction protocols recently demonstrated in diamond. However,