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We consider the degree of conservation of nuclear spin polarization in the process of optical pumping under typical spin-exchange optical pumping conditions. Previous analyses have assumed that negligible nuclear spin precession occurs in the brief periods of time the alkali-metal atoms are in the excited state after absorbing photons and before undergoing quenching collisions with nitrogen molecules. We include excited-state hyperfine interactions, electronic spin relaxation in collisions with He and N_2, spontaneous emission, quenching collisions, and a simplified treatment of radiation trapping.
We have observed depolarization effects when high intensity cold neutron beams are incident on alkali-metal-spin-exchange polarized He-3 cells used as neutron spin filters. This was first observed as a reduction of the maximum attainable He-3 polariz
We report high steady-state nuclear polarization of 1 torr $^3$He gas nuclei via metastability-exchange optical pumping at magnetic fields above 2 T. The introduction of highly polarized $^3$He gas into Brookhavens Electron Beam Ion Source would enab
The Zeeman splittings and EPR frequencies of alkali-metal atoms are shifted in the presence of a polarized noble gas. For a spherical geometry, the shift is enhanced over what is expected classically by a dimensionless atomic parameter $kappa_0$ that
We report on hyperpolarization of quadrupolar (I=3/2) 131Xe via spin-exchange optical pumping. Observations of the 131Xe polarization dynamics show that the effective alkali-metal/131Xe spin-exchange cross-sections are large enough to compete with 13
We measure the ratio $gamma$ of the momentum-transfer to the vibrational quenching cross section for the X ($^1Sigma^+$), $ u=1$, $mathrm{J=0}$ state of molecular thorium monoxide (ThO) in collisions with atomic $^3$He between 800 mK and 2.4 K. We ob