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The main obstacle to coherent control of two-level quantum systems is their coupling to an uncontrolled environment. For electron spins in III-V quantum dots, the random environment is mostly given by the nuclear spins in the quantum dot host material; they collectively act on the electron spin through the hyperfine interaction, much like a random magnetic field. Here we show that the same hyperfine interaction can be harnessed such that partial control of the normally uncontrolled environment becomes possible. In particular, we observe that the electron spin resonance frequency remains locked to the frequency of an applied microwave magnetic field, even when the external magnetic field or the excitation frequency are changed. The nuclear field thereby adjusts itself such that the electron spin resonance condition remains satisfied. General theoretical arguments indicate that this spin resonance locking is accompanied by a significant reduction of the randomness in the nuclear field.
We show that scattering of the conduction electrons by nuclear spins via the hyperfine interaction may lead the upper limit on the mean free path in clean metals. Nuclear spins with s >1/2 may cause a strong dephasing in dirty limit due to the quadru
We polarize nuclear spins in a GaAs double quantum dot by controlling two-electron spin states near the anti-crossing of the singlet (S) and m_S=+1 triplet (T+) using pulsed gates. An initialized S state is cyclically brought into resonance with the
We show here the existence of the indirect coupling of electron and magnetic or nuclear ion spins in self-assembled quantum dots mediated by electron-electron interactions. With a single localized spin placed in the center of the dot, only the spins
We experimentally demonstrate the use of a single electronic spin to measure the quantum dynamics of distant individual nuclear spins from within a surrounding spin bath. Our technique exploits coherent control of the electron spin, allowing us to is
We study decoherence of nuclear spins in a GaAs quantum well structure using resistively detected nuclear magnetic resonance. The transverse decoherence time T2 of 75As nuclei is estimated from Rabi-type coherent oscillations as well as by using spin