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تسجيل مستخدم جديدStructure and superconductivity of LiFeAs
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The lithium ions in Lithium iron arsenide phases with compositions close to LiFeAs have been located using powder neutron diffraction. These phases exhibit superconductivity at temperatures at least as high as 16 K demonstrating that superconductivity in compounds with [FeAs]- anti-PbO-type anionic layers occurs in compounds with at least three different structure types and occurs for a wide range of As-Fe-As bond angles.
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We measured the optical conductivity of superconducting LiFeAs. In the superconducting state, the formation of the condensate leads to a spectral-weight loss and yields a penetration depth of 225 nm. No sharp signature of the superconducting gap is o
bserved. This suggests that the system is likely in the clean limit. A Drude-Lorentz parametrization of the data in the normal state reveals a quasiparticle scattering rate supportive of spin fluctuations and proximity to a quantum critical point.
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A new iron arsenide superconducting system LiFeAs was found that crystallizes into a tetragonal structure with space group P4/nmm. The superconductivity with Tc up to 18 K was observed in the compounds. This simple 111 type layered iron arsenide supe
rconductor can be viewed as an analogue of the infinite layer structure of copper oxides.
Multiorbital models are important to both the correlation physics and topological behavior of quantum materials. LiFeAs is a prototype iron pnictide suitable for indepth investigation of this issue. Its electronic structure is strikingly different fr
om the prediction of the noninteracting description. Here, a multiorbital Hubbard model for this compound is studied using a $U(1)$ slave spin theory. We demonstrate a new mechanism for a large change in the size of the Fermi surface, namely, orbital selectivity of the energy-level renormalization cooperating with its counterpart in the quasiparticle spectral weight. Using this effect, we show how the dominating features of the electronic structure in LiFeAs are understood in terms of the local correlations alone. Our results reveal a remarkable degree of universality out of the seemingly complex multiorbital building blocks across a broad range of strongly correlated superconductors.
If strong electron-electron interactions between neighboring Fe atoms mediate the Cooper pairing in iron-pnictide superconductors, then specific and distinct anisotropic superconducting energy gaps Delta_i(k) should appear on the different electronic
bands i. Here we introduce intra-band Bogoliubov quasiparticle scattering interference (QPI) techniques for determination of Delta_i(k) in such materials, focusing on LiFeAs. We identify the three hole-like bands assigned previously as gamma, alpha_2 and alpha_1, and we determine the anisotropy, magnitude and relative orientations of their Delta_i(k). These measurements will advance quantitative theoretical analysis of the mechanism of Cooper pairing in iron-based superconductivity.
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