ترغب بنشر مسار تعليمي؟ اضغط هنا

MuSR and SQUID Investigation of Superconductivity in (NH_3)_0.75NaK_2C_60

412   0   0.0 ( 0 )
 نشر من قبل Toni Shiroka
 تاريخ النشر 2002
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

The family of superconducting fullerides (NH_3)_xNaK_2C_60 shows an anomalous correlation between T_c and lattice parameter. To better understand the origin of this anomaly we have studied a representative x=0.75 compound using SQUID magnetometry and MuSR spectroscopy. The lower critical field H_c1, measured by the trapped magnetization method, is less than 1 G, a very small value as compared with that of other fullerides. Muon spin depolarization in the superconducting phase shows also quite small local field inhomogeneities, of the order of those arising from nuclear dipolar fields. On the other hand, the 40 T value for H_c2, as extracted from magnetometry data, is comparable to that of other fullerides. We show that these observations cannot be rationalized within the framework of the Ginzburg-Landau theory of superconductivity. Instead, the anomalous magnetic properties could be interpreted taking into account the role played by polaronic instabilities in this material.



قيم البحث

اقرأ أيضاً

The discovery of superconductivity in Sr-doped NdNiO$_{2}$ is a crucial breakthrough in the long pursuit for nickel oxide materials with electronic and magnetic properties similar to those of the cuprates. NdNiO$_2$ is the infinite-layer member of a family of square-planar nickelates with general chemical formula R$_{n+1}$Ni$_n$O$_{2n+2}$ (R = La, Pr, Nd, $n= 2, 3, ... infty$). In this letter, we investigate superconductivity in the trilayer member of this series (R$_4$Ni$_3$O$_8$) using a combination of first-principles and $t-J$ model calculations. R$_4$Ni$_3$O$_8$ compounds resemble cuprates more than RNiO$_2$ materials in that only Ni-$d_{x^{2}-y^{2}}$ bands cross the Fermi level, they exhibit a largely reduced charge transfer energy, and as a consequence superexchange interactions are significantly enhanced. We find that the superconducting instability in doped R$_4$Ni$_3$O$_8$ compounds is considerably stronger with a maximum gap about four times larger than that in Sr$_{0.2}$Nd$_{0.8}$NiO$_2$.
The superconducting properties of the recently discovered double Fe$_2$As$_2$ layered high-$T_c$ superconductor RbCa$_2$Fe$_4$As$_4$F$_2$ with $T_capprox$ 30~K have been investigated using magnetization, heat capacity, transverse-field (TF) and zero- field (ZF) muon-spin rotation/relaxation ($mu$SR) measurements. Our low field magnetization measurements and heat capacity (C$_p$) reveal an onset of bulk superconductivity with $T_{bf c}sim$ 30.0(4) K. Furthermore, the heat capacity exhibits a jump at $T_{bf c}$ of $Delta$C$_p$/$T_{bf c}$=94.6 (mJ/mole-K$^2$) and no clear effect of applied magnetic fields was observed on C$_p$(T) up to 9 T between 2 K and 5 K. Our analysis of the TF-$mu$SR results shows that the temperature dependence of the magnetic penetration depth is better described by a two-gap model, either isotropic $s$+$s$-wave or $s$+$d$-wave than a single gap isotropic $s$-wave or $d$-wave model for the superconducting gap. The presence of two superconducting gaps in RbCa$_2$Fe$_4$As$_4$F$_2$ suggests a multiband nature of the superconductivity, which is consistent with the multigap superconductivity observed in other Fe-based superconductors, including ACa$_2$Fe$_4$As$_4$F$_2$ (A=K and Cs). Furthermore, from our TF-$mu$SR study we have estimated an in-plane penetration depth $lambda_{mathrm{ab}}$$(0)$ =231.5(3) nm, superconducting carrier density $n_s = 7.45 times 10^{26}~ $m$^{-3}$, and carriers effective-mass $m^*$ = 2.45textit{m}$_{e}$. Our ZF $mu$SR measurements do not reveal a clear sign of time reversal symmetry breaking at $T_{bf c}$, but the temperature dependent relaxation between 150 K and 1.2 K might indicate the presence of spin-fluctuations. The results of our present study have been compared with those reported for other Fe pnictide superconductors.
We have investigated the bulk and microscopic properties of the rhombohedral intermediate valence superconductor CeIr$_3$ by employing magnetization, heat capacity, and muon spin rotation and relaxation ($mu$SR) measurements. The magnetic susceptibil ity indicates bulk superconductivity below $T_mathrm{C} = 3.1$~K. Heat capacity data also reveal a bulk superconducting transition at $T_mathrm{C} = 3.1$~K with a second weak anomaly near 1.6~K. At $T_{mathrm{C}}$, the jump in heat capacity $Delta C$/$gamma T_{mathrm{C}} sim 1.39(1)$, is slightly less than the BCS weak coupling limit of 1.43. Transverse-field $mu$SR measurements suggest a fully gapped, isotropic, $s$-wave superconductivity with 2$Delta(0)/k_{mathrm{B}}T_{mathrm{C}} = 3.76(3)$, very close to 3.56, the BCS gap value for weak-coupling superconductors. From the temperature variation of magnetic penetration depth, we have also determined the London penetration depth $lambda_{mathrm{L}}(0) = 435(2)$~nm, the carriers effective mass enhancement $m^{*} = 1.69(1)m_{mathrm{e}}$ and the superconducting carrier density $n_{mathrm{s}} = 2.5(1)times 10^{26}$ carriers m$^{-3}$. The fact that LaIr$_3$, with no $4f$-electrons, and CeIr$_3$ with $4f^{n}$ electrons where $n le 1$-electron (Ce ion in a valence fluctuating state), both exhibit the same $s$-wave gap symmetry indicates that the physics of these two compounds is governed by the Ir-$d$ band near the Fermi-level, which is in agreement with previous band structure calculations.
The compound Sr$_{0.5}$Ce$_{0.5}$FBiS$_{2}$ belongs to the intensively studied family of layered BiS$_2$ superconductors. It attracts special attention because superconductivity at $T_{sc} = 2.8$ K was found to coexist with local-moment ferromagnetic order with a Curie temperature $T_C = 7.5$ K. Recently it was reported that upon replacing S by Se $T_C$ drops and ferromagnetism becomes of an itinerant nature (Thakur et al., Sci. Reports 6, 37527 (2016)). At the same time $T_{sc}$ increases and it was argued superconductivity coexists with itinerant ferromagnetism. Here we report a muon spin rotation and relaxation study ($mu$SR) conducted to investigate the coexistence of superconductivity and ferromagnetic order in Sr$_{0.5}$Ce$_{0.5}$FBiS$_{2-x}$Se$_x$ with $x=0.5$ and $1.0$. By inspecting the muon asymmetry function we find that both phases do not coexist on the microscopic scale, but occupy different sample volumes. For $x=0.5$ and $x=1.0$ we find a ferromagnetic volume fraction of $sim , 8 %$ and $sim , 30 %$ at $T=0.25$ K, well below $T_{C} = 3.4$ K and $T_C = 3.3$ K, respectively. For $x=1.0$ ($T_{sc} = 2.9$ K) the superconducting phase occupies the remaining sample volume ($sim , 70 %$), as shown by transverse field experiments that probe the Gaussian damping due to the vortex lattice. We conclude ferromagnetism and superconductivity are macroscopically phase separated.
We use muon spin relaxation (muSR) to investigate the magnetic properties of a bulk form diluted ferromagnetic semiconductor (DFS) Li1.15(Zn0.9Mn0.1)P with T_C ~ 22 K. MuSR results confirm the gradual development of ferromagnetic ordering below T_C w ith a nearly 100% magnetic ordered volume. Despite its low carrier density, the relation between static internal field and Curie temperature observed for Li(Zn,Mn)P is consistent with the trend found in (Ga,Mn)As and other bulk DFSs, indicating these systems share a common mechanism for the ferromagnetic exchange interaction. Li1+y(Zn1-xMnx)P has the advantage of decoupled carrier and spin doping, where Mn2+ substitution for Zn2+ introduces spins and Li+ off-stoichiometry provides carriers. This advantage enables us to investigate the influence of overdoped Li on the ferromagnetic ordered state. Overdoping Li suppresses both T_C and saturation moments for a certain amount of spins, which indicates that more carriers are detrimental to the ferromagnetic exchange interaction, and that a delicate balance between charge and spin densities is required to achieve highest T_C.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا