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We study an atomic comagnetometer design based on the spin precessions of $^{129}$Xe and $^{131}$Xe atoms in glass cells. The quadrupole splittings in the precession spectrum of $^{131}$Xe are fully resolved, allowing a precise determination of the magnetic-dipole precession frequency. The transverse asymmetry of quadrupole interactions, due to both the geometry and surface properties of the cell, characterized by a non-zero asymmetry parameter $eta$, modifies the dependence of the quadrupole splittings on the relative orientation between the cell axes and the bias magnetic field, and lead to additional corrections in the precession frequencies of $^{131}$Xe atoms. We examine these effects both theoretically and experimentally, and develop methods to quantify and control such shifts.
We report on the operation of co-located ${}^{129}$Xe and ${}^{131}$Xe nuclear spin masers with an external feedback scheme, and discuss the use of ${}^{131}$Xe as a comagnetometer in measurements of the ${}^{129}$Xe spin precession frequency. By app
We report the observation of dipole-forbidden, but quadrupole-allowed, one-photon transitions to high Rydberg states in Rb. Using pulsed UV excitation of ultracold atoms in a magneto-optical trap, we excite $5s to nd$ transitions over a range of prin
Recent advances in the high sensitivity spectroscopy have made it possible, in combination with accurate theoretical predictions, to observe for the first time very weak electric quadrupole transitions in a polar polyatomic molecule of water. Here we
We report on a new measurement of the CP-violating permanent Electric Dipole Moment (EDM) of the neutral $^{129}$Xe atom. Our experimental approach is based on the detection of the free precession of co-located nuclear spin-polarized $^3$He and $^{12
We report experimental results on the first on-sky observation of atomic spin precession of mesospheric sodium driven by polarization modulation of a continuous-wave laser. The magnetic resonance was remotely detected from the ground by observing the