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In the quest to image the three-dimensional magnetization structure we show that the technique of magnetic small-angle neutron scattering (SANS) is highly sensitive to the details of the internal spin structure of nanoparticles. By combining SANS with numerical micromagnetic computations we study the transition from single-domain to multi-domain behavior in nanoparticles and its implications for the ensuing magnetic SANS cross section. Above the critical single-domain size we find that the cross section and the related correlation function cannot be described anymore with the uniform particle model, resulting e.g. in deviations from the well-known Guinier law. We identify a clear signature for the occurrence of a vortex-like spin structure at remanence. The micromagnetic approach to magnetic SANS bears great potential for future investigations, since it provides fundamental insights into the mesoscale magnetization profile of nanoparticles.
The scientific and technological exploration of artificially designed three-dimensional magnetic nanostructures opens the path to exciting novel physical phenomena, originating from the increased complexity in spin textures, topology, and frustration
An experimentally feasible energy-storage concept is formulated based on vorticity (hydro)dynamics within an easy-plane insulating magnet. The free energy, associated with the magnetic winding texture, is built up in a circular easy-plane magnetic st
We performed high resolution diffraction and inelastic neutron scattering measurements of Mn_{12}-acetate. Using a very high energy resolution, we could separate the energy levels corresponding to the splitting of the lowest S multiplet. Data were an
We provide a general procedure to calculate the current-induced spin-transfer torque which acts on a general steep magnetic texture due to the exchange interaction with an applied spin-polarized current. As an example, we consider a one-dimensional f
The physical characterisation and understanding of molecular magnetic materials is one of the most important steps towards the integration of such systems in hybrid spintronic devices. Amongst the many characterisation techniques employed in such a t