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Magnetometry utilizing a spin qubit in a solid state possesses high sensitivity. In particular, a magnetic sensor with a high spatial resolution can be achieved with the electron-spin states of a nitrogen vacancy (NV) center in diamond. In this study, we demonstrated that NV quantum sensing based on multiple-pulse decoupling sequences can sensitively measure not only the amplitude but also the phase shift of an alternating-current (AC) magnetic field. In the AC magnetometry based on decoupling sequences, the maximum phase accumulation of the NV spin due to an AC field can be generally obtained when the $pi$-pulse period in the sequences matches the half time period of the field and the relative phase difference between the sequences and the field is zero. By contrast, the NV quantum sensor acquires no phase accumulation if the relative phase difference is $pi/2$. Thus, this phase-accumulation condition does not have any advantage for the magnetometry. However, we revealed that the non-phase-accumulation condition is available for detecting a very small phase shift of an AC field from its initial phase. This finding is expected to provide a guide for realizing sensitive measurement of a complex AC magnetic field in micrometer and nanometer scales.
Multipulse sequences based on Carr-Purcell decoupling are frequently used for narrow-band signal detection in single spin magnetometry. We have analyzed the behavior of multipulse sensing sequences under real-world conditions, including finite pulse
Sensing the internal dynamics of individual nuclear spins or clusters of nuclear spins has recently become possible by observing the coherence decay of a nearby electronic spin: the weak magnetic noise is amplified by a periodic, multi-pulse decoupli
A solid state spin is an attractive system with which to realize an ultra-sensitive magnetic field sensor. A spin superposition state will acquire a phase induced by the target field, and we can estimate the field strength from this phase. Recent stu
Even though the traditional dynamical decoupling methods have the ability to resist dynamic dephasing caused by low frequency noise, they are not appropriate for suppressing the residual geometric dephasing, which arises from the disturbance for the
Quantum sensing exploits the strong sensitivity of quantum systems to measure small external signals. The nitrogen-vacancy (NV) center in diamond is one of the most promising platforms for real-world quantum sensing applications, predominantly used a