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The coherent high-fidelity generation of nuclear spins in long-lived singlet states which may find application as quantum memory or sensor represents a considerable experimental challenge. Here we propose a dissipative scheme that achieves the preparation of pairs of nuclear spins in long-lived singlet states by a protocol that combines the interaction between the nuclei and a periodically reset electron spin of an NV center with local rf-control of the nuclear spins. The final state of this protocol is independent of the initial preparation of the nuclei, is robust to external field fluctuations and can be operated at room temperature. We show that a high fidelity singlet pair of a 13C dimer in a nuclear bath in diamond can be generated under realistic experimental conditions.
We introduce a broadly applicable technique to create nuclear spin singlet states in organic molecules and other many-atom systems. We employ a novel pulse sequence to produce a spin-lock induced crossing (SLIC) of the spin singlet and triplet energy
We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an off-axis ma
We probe small scalar coupling differences via the coherent interactions between two nuclear spin singlet states in organic molecules. We show that the spin-lock induced crossing (SLIC) technique enables the coherent transfer of singlet order between
Quantum memories provide intermediate storage of quantum information until it is needed for the next step of a quantum algorithm or a quantum communication process. Relevant figures of merit are therefore the fidelity with which the information can b
There has been much recent interest in long-lived massive particles at the LHC, understood as those with lifetimes between tens of micrometers and several meters. In this context we consider the possibility of long-lived electroweak singlet scalars c