ترغب بنشر مسار تعليمي؟ اضغط هنا

Coulomb mediated hybridization of excitons in artificial molecules

65   0   0.0 ( 0 )
 نشر من قبل Per-Lennart Ardelt
 تاريخ النشر 2015
  مجال البحث فيزياء
والبحث باللغة English




اسأل ChatGPT حول البحث

We report the Coulomb mediated hybridization of excitonic states in an optically active, artificial quantum dot molecule. By probing the optical response of the artificial molecule as a function of the static electric field applied along the molecular axis, we observe unexpected avoided level crossings that do not arise from the dominant single particle tunnel coupling. We identify a new few-particle coupling mechanism stemming from Coulomb interactions between different neutral exciton states. Such Coulomb resonances hybridize the exciton wave function over four different electron and hole single-particle orbitals. Comparisons of experimental observations with microscopic 8-band $k cdot p$ calculations taking into account a realistic quantum dot geometry show good agreement and reveal that the Coulomb resonances arise from broken symmetry in the artificial molecule.



قيم البحث

اقرأ أيضاً

The many-body state of carriers confined in a quantum dot is controlled by the balance between their kinetic energy and their Coulomb correlation. In coupled quantum dots, both can be tuned by varying the inter-dot tunneling and interactions. Using a theoretical approach based on the diagonalization of the exact Hamiltonian, we show that transitions between different quantum phases can be induced through inter-dot coupling both for a system of few electrons (or holes) and for aggregates of electrons and holes. We discuss their manifestations in addition energy spectra (accessible through capacitance or transport experiments) and optical spectra.
121 - Zhien Lu , Ka-di Zhu 2008
The optical properties of hybrid molecules composed of semiconductor and metal nanoparticles with a weak probe in a strong pump field are investigated theoretically. Excitons in such a hybrid molecule demonstrate novel optical properties due to the c oupling between exciton and plasmon. It is shown that a non-absorption hole induced by coherent population oscillation appears at the absorption spectrum of the probe field and there exists slow light effect resulting in the great change of the refractive index. The numerical results indicate that with the different center-to-center distance between the two nanopaticles the slow light effects are greatly modified in terms of exciton-plasmon couplings.
We analyze theoretically the Coulomb scattering processes of highly excited excitons in the direct bandgap semiconductor quantum wells. We find that contrary to the interaction of ground state excitons the electron and hole exchange interaction betwe en excited excitons has an attractive character both for $s$- and $p$-type 2D excitons. Moreover, we show that similarly to the three-dimensional (3D) highly excited excitons, the direct interaction of 2D Rydberg excitons exhibits van der Waals type long-range interaction. The results predict the linear growth of the absolute value of exchange interaction strength with an exciton principal quantum number, and point the way towards enhancement of optical nonlinearity in 2D excitonic systems.
Using wide spectral range in situ spectroscopic ellipsometry with systematic ultra high vacuum annealing and in situ exposure to oxygen, we report the complex dielectric function of MoS$_2$ isolating the environmental effects and revealing the crucia l role of unpassivated and passivated sulphur vacancies. The spectral weights of the A ($1.92$ eV) and B ($2.02$ eV) exciton peaks in the dielectric function reduce significantly upon annealing, accompanied by spectral weight transfer in a broad energy range. Interestingly, the original spectral weights are recovered upon controlled oxygen exposure. This tunability of the excitonic effects is likely due to passivation and reemergence of the gap states in the bandstructure during oxygen adsorption and desorption, respectively, as indicated by ab initio density functional theory calculation results. This work unravels and emphasizes the important role of adsorbed oxygen in the optical spectra and many-body interactions of MoS$_2$.
We address the electronically induced anisotropy field acting on a spin moment comprised in a vibrating magnetic molecule located in the junction between ferromagnetic metals. Under weak coupling between the electrons and molecular vibrations, the na ture of the anisotropy can be changed from favoring a high spin (easy axis) magnetic moment to a low spin (easy plane) by applying a temperature difference or a voltage bias across the junction. For unequal spin-polarizations in the ferromagnetic metals it is shown that the character of the anisotropy is essentially determined by the properties of the weaker ferromagnet. By increasing the temperature in this metal, or introducing a voltage bias, its influence can be suppressed such that the dominant contribution to the anisotropy is interchanged to the stronger ferromagnet. With increasing coupling strength between the molecular vibrations and the electrons, the nature of the anisotropy is locked into favoring easy plane magnetism.
التعليقات
جاري جلب التعليقات جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا