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تسجيل مستخدم جديدFermi-surface topological phase transition and horizontal order-parameter nodes in CaFe$_2$As$_2$ under pressure
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Iron-based compounds (IBS) display a surprising variety of superconducting properties that seems to arise from the strong sensitivity of these systems to tiny details of the lattice structure. In this respect, systems that become superconducting under pressure, like CaFe$_2$As$_2$, are of particular interest. Here we report on the first directional point-contact Andreev-reflection spectroscopy (PCARS) measurements on CaFe$_2$As$_2$ crystals under quasi-hydrostatic pressure, and on the interpretation of the results using a 3D model for Andreev reflection combined with ab-initio calculations of the Fermi surface (within the density functional theory) and of the order parameter symmetry (within a random-phase-approximation approach in a ten-orbital model). The almost perfect agreement between PCARS results at different pressures and theoretical predictions highlights the intimate connection between the changes in the lattice structure, a topological transition in the hole-like Fermi surface sheet, and the emergence on the same sheet of an order parameter with a horizontal node line.
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CaFe$_2$As$_2$ has been synthesized and found to form in the tetragonal, ThCr$_2$Si$_2$ structure with lattice parameters $a = 3.912(68) AA$ and $c = 11.667(45) AA$. Upon cooling through 170 K, CaFe$_2$As$_2$ undergoes a first order, structural phase
transition to a low temperature, orthorhombic phase with a $2 - 3$ K range of hysteresis and coexistence. This transition is clearly evident in microscopic, thermodynamic and transport measurements. CaFe$_2$As$_2$ is the third member of the AFe$_2$As$_2$ (A = Ba, Sr, Ca) family to exhibit such a dramatic phase transition and is a promising candidate for studies of doping induced superconductivity.
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We reexamined the experimental evidences for the possible existence of the superconducting (SC) gap nodes in the three most suspected Fe-pnictide SC compounds: LaFePO, BaFe$_2$(As$_{0.67}$P$_{0.33}$)$_2$, and KFe$_2$As$_2$. We showed that while the $
T$-linear temperature dependence of the penetration depth $lambda(T)$ of these three compounds indicate extremely clean nodal gap superconductors, the thermal conductivity data $lim_{T,H rightarrow 0} kappa_S (H,T)/T$ unambiguously showed that LaFePO and BaFe$_2$(As$_{0.67}$P$_{0.33}$)$_2$ are extremely dirty, while KFe$_2$As$_2$ can be clean. This apparently conflicting experimental data casts a serious doubt on the nodal gap possibility on LaFePO and BaFe$_2$(As$_{0.67}$P$_{0.33}$)$_2$.
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