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Realizing a strong interaction between individual optical photons is an important objective of research in quantum science and technology. Since photons do not interact directly, this goal requires, e.g., an optical medium in which the light experiences a phase shift that depends nonlinearly on the photon number. Once the additional phase shift for two photons reaches pi, such an ultra-strong nonlinearity could even enable the direct implementation of high-fidelity quantum logic operations. However, the nonlinear response of standard optical media is many orders of magnitude too weak for this task. Here, we demonstrate the realization of an optical fiber-based nonlinearity that leads to an additional two-photon phase shift close to the ideal value of pi. Our scheme employs a whispering-gallery-mode resonator, interfaced by an optical nanofiber, where the presence of a single rubidium atom in the resonator results in a strongly nonlinear response. We experimentally show that this results in entanglement of initially independent incident photons. The demonstration of this ultra-strong nonlinearity in a fiber-integrated system is a decisive step towards scalable quantum logics with optical photons.
We report on a direct measurement of a phase shift on a weak coherent beam by a single Rb-87 atom in a Mach-Zehnder interferometer. A maximum phase shift of about 1 degree is observed experimentally.
We succeeded in measuring phase shift spectra of a microsphere cavity coupled with a tapered fiber using a weak coherent probe light at the single photon level. We utilized a tapered fiber with almost no depolarization and constructed a very stable p
In analogy to transistors in classical electronic circuits, a quantum optical switch is an important element of quantum circuits and quantum networks. Operated at the fundamental limit where a single quantum of light or matter controls another field
It has been suggested that second-order nonlinearities could be used for quantum logic at the single-photon level. Specifically, successive two-photon processes in principle could accomplish the phase shift (conditioned on the presence of two photons
A diamond nano-crystal hosting a single nitrogen vacancy (NV) center is optically selected with a confocal scanning microscope and positioned deterministically onto the subwavelength-diameter waist of a tapered optical fiber (TOF) with the help of an