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We report a measurement on the temporal response of a plasmonic antenna at the femtosecond time scale. The antenna consists of a square array of nanometer-size gold rods. We find that the far-field dispersion of light reflected from the plasmonic antenna is less than that of a 1.2 mm thick glass slide. Assuming a simple oscillating dipole model this implies that the near-field of the antenna may be used as an electron switch that responds faster than 20 fs. Alternatively, ultrafast electron diffraction may be used to investigate the near-field dynamics of the plasmonic antenna.
We investigate the chiroptical response of a single plasmonic nanohelix interacting with a weakly-focused circularly-polarized Gaussian beam. The optical scattering at the fundamental resonance is characterized experimentally, and the chiral behavior
Efficient frequency conversion techniques are crucial to the development of plasmonic metasurfaces for information processing and signal modulation. In principle, nanoscale electric-field confinement in nonlinear materials enables higher harmonic con
Starting from first principles, we theoretically model the nonlinear temporal dynamics of gold-based plasmonic devices resulting from the heating of their metallic components. At optical frequencies, the gold susceptibility is determined by the inter
The nonlinear optical response of materials to exciting light is enhanced by resonances between the incident laser frequencies and the energy levels of the excited material. Traditionally, in molecular nonlinear spectroscopy one tunes the input laser
Femtosecond-scale polarization state conversion is experimentally found in optical response of a plasmonic nanograting by means of time-resolved polarimetry. Simultaneous measurements of the Stokes parameters as a function of time with an averaging t