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تسجيل مستخدم جديدAdvances in Atomic Data for Neutron-Capture Elements
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تأليف
N. C. Sterling
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Neutron(n)-capture elements (atomic number Z>30), which can be produced in planetary nebula (PN) progenitor stars via s-process nucleosynthesis, have been detected in nearly 100 PNe. This demonstrates that nebular spectroscopy is a potentially powerful tool for studying the production and chemical evolution of trans-iron elements. However, significant challenges must be addressed before this goal can be achieved. One of the most substantial hurdles is the lack of atomic data for n-capture elements, particularly that needed to solve for their ionization equilibrium (and hence to convert ionic abundances to elemental abundances). To address this need, we have computed photoionization cross sections and radiative and dielectronic recombination rate coefficients for the first six ions of Se and Kr. The calculations were benchmarked against experimental photoionization cross section measurements. In addition, we computed charge transfer (CT) rate coefficients for ions of six n-capture elements. These efforts will enable the accurate determination of nebular Se and Kr abundances, allowing robust investigations of s-process enrichments in PNe.
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We present multi-configuration Breit-Pauli AUTOSTRUCTURE calculations of distorted-wave photoionization (PI) cross sections, and total and partial final-state resolved radiative recombination (RR) and dielectronic recombination (DR) rate coefficients
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We present multi-configuration Breit-Pauli distorted-wave photoionization (PI) cross sections and radiative recombination (RR) and dielectronic recombination (DR) rate coefficients for the first six krypton ions. These were calculated with the AUTOST
RUCTURE code, using semi-relativistic radial wavefunctions in intermediate coupling. Kr has been detected in several planetary nebulae (PNe) and H II regions, and is a useful tracer of neutron-capture nucleosynthesis. PI, RR, and DR data are required to accurately correct for unobserved Kr ions in ionized nebulae, and hence to determine elemental Kr abundances. PI cross sections have been determined for ground configuration states of Kr^0--Kr^5+ up to 100 Rydbergs. Our Kr^+ PI calculations were significantly improved through comparison with experimental measurements. RR and DR rate coefficients were determined from the direct and resonant PI cross sections at temperatures (10^1--10^7)z^2 K, where z is the charge. We account for Delta n=0 DR core excitations, and find that DR is the dominant recombination mechanism for all but Kr^+ at photoionized plasma temperatures. Internal uncertainties are estimated by comparing results computed with three different configuration-interaction expansions for each ion, and by testing the sensitivity to variations in the orbital radial scaling parameters. The PI cross sections are generally uncertain by 30-50% near the ground state thresholds. Near 10^4 K, the RR rate coefficients are typically uncertain by <10%, while those of DR exhibit uncertainties of factors of 2 to 3, due to the unknown energies of near-threshold autoionizing resonances. With the charge transfer rate coefficients presented in the third paper of this series, these data enable robust Kr abundance determinations in photoionized nebulae for the first time.
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