اشترك بالحزمة الذهبية واحصل على وصول غير محدود شمرا أكاديميا
تسجيل مستخدم جديدThermal effects in exciton harvesting in biased one-dimensional systems
105
0
0.0
(
0
)
اسأل ChatGPT حول البحث
ﻻ يوجد ملخص باللغة العربية
The study of energy harvesting in chain-like structures is important due to its relevance to a variety of interesting physical systems. Harvesting is understood as the combination of exciton transport through intra-band exciton relaxation (via scattering on phonon modes) and subsequent quenching by a trap. Previously, we have shown that in the low temperature limit different harvesting scenarios as a function of the applied bias strength (slope of the energy gradient towards the trap) are possible cite{Vlaming07}. This paper generalizes the results for both homogeneous and disordered chains to nonzero temperatures. We show that thermal effects are appreciable only for low bias strengths, particularly so in disordered systems, and lead to faster harvesting.
قيم البحث
اقرأ أيضاً
We theoretically study the efficiency of energy harvesting in linear exciton chains with an energy bias, where the initial excitation is taking place at the high-energy end of the chain and the energy is harvested (trapped) at the other end. The effi
ciency is characterized by means of the average time for the exciton to be trapped after the initial excitation. The exciton transport is treated as the intraband energy relaxation over the states obtained by numerically diagonalizing the Frenkel Hamiltonian that corresponds to the biased chain. The relevant intraband scattering rates are obtained from a linear exciton-phonon interaction. Numerical solution of the Pauli master equation that describes the relaxation and trapping processes, reveals a complicated interplay of factors that determine the overall harvesting efficiency. Specifically, if the trapping step is slower than or comparable to the intraband relaxation, this efficiency shows a nonmonotonic dependence on the bias: it first increases when introducing a bias, reaches a maximum at an optimal bias value, and then decreases again because of dynamic (Bloch) localization of the exciton states. Effects of on-site (diagonal) disorder, leading to Anderson localization, are addressed as well.
The transport of excitations between pinned particles in many physical systems may be mapped to single-particle models with power-law hopping, $1/r^a$. For randomly spaced particles, these models present an effective peculiar disorder that leads to s
urprising localization properties. We show that in one-dimensional systems almost all eigenstates (except for a few states close to the ground state) are power-law localized for any value of $a>0$. Moreover, we show that our model is an example of a new universality class of models with power-law hopping, characterized by a duality between systems with long-range hops ($a<1$) and short-range hops ($a>1$) in which the wave function amplitude falls off algebraically with the same power $gamma$ from the localization center.
In the conventional theory of hopping transport the positions of localized electronic states are assumed to be fixed, and thermal fluctuations of atoms enter the theory only through the notion of phonons. On the other hand, in 1D and 2D lattices, whe
re fluctuations prevent formation of long-range order, the motion of atoms has the character of the large scale diffusion. In this case the picture of static localized sites may be inadequate. We argue that for a certain range of parameters, hopping of charge carriers among localization sites in a network of 1D chains is a much slower process than diffusion of the sites themselves. Then the carriers move through the network transported along the chains by mobile localization sites jumping occasionally between the chains. This mechanism may result in temperature independent mobility and frequency dependence similar to that for conventional hopping.
We study anomalous transport arising in disordered one-dimensional spin chains, specifically focusing on the subdiffusive transport typically found in a phase preceding the many-body localization transition. Different types of transport can be distin
guished by the scaling of the average resistance with the systems length. We address the following question: what is the distribution of resistance over different disorder realizations, and how does it differ between transport types? In particular, an often evoked so-called Griffiths picture, that aims to explain slow transport as being due to rare regions of high disorder, would predict that the diverging resistivity is due to fat power-law tails in the resistance distribution. Studying many-particle systems with and without interactions we do not find any clear signs of fat tails. The data is compatible with distributions that decay faster than any power law required by the fat tails scenario. Among the distributions compatible with the data, a simple additivity argument suggests a Gaussian distribution for a fractional power of the resistance.
We study heat conduction mediated by longitudinal phonons in one dimensional disordered harmonic chains. Using scaling properties of the phonon density of states and localization in disordered systems, we find non-trivial scaling of the thermal condu
ctance with the system size. Our findings are corroborated by extensive numerical analysis. We show that a system with strong disorder, characterized by a `heavy-tailed probability distribution, and with large impedance mismatch between the bath and the system satisfies Fouriers law. We identify a dimensionless scaling parameter, related to the temperature scale and the localization length of the phonons, through which the thermal conductance for different models of disorder and different temperatures follows a universal behavior.
سجل دخول لتتمكن من نشر تعليقات
التعليقات
جاري جلب التعليقات
سجل دخول لتتمكن من متابعة معايير البحث التي قمت باختيارها
