In the present paper, we construct spontaneously scalarized rotating black hole solutions in dynamical Chern-Simons (dCS) gravity by following the scalar field evolution in the decoupling limit. For the range of parameters where the Kerr black hole becomes unstable within dCS gravity the scalar field grows exponentially until it reaches an equilibrium configuration that is independent of the initial perturbation. Interestingly, the $mathbb{Z}_2$ symmetry of the scalar field is broken and a strong maximum around only one of the rotational axes can be observed. The black hole scalar charge is calculated for two coupling functions suggesting that the main observations would remain qualitatively correct even if one considers coupling functions/coupling parameters producing large deviations from the Kerr solution beyond the decoupling limit approximation.
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