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Register a new userEnergy Sharing in the 2-Electron Attosecond Streak Camera
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Added by
Agapi Emmanouilidou
Publication date
2011
fields
Physics
and research's language is
English
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Using the recently developed concept of the 2-electron streak camera (see NJP 12, 103024 (2010)), we have studied the energy-sharing between the two ionizing electrons in single-photon double ionization of He(1s2s). We find that the most symmetric and asymmetric energy sharings correspond to different ionization dynamics with the ions Coulomb potential significantly influencing the latter. This different dynamics for the two extreme energy sharings gives rise to different patterns in asymptotic observables and different time-delays between the emission of the two electrons. We show that the 2-electron streak camera resolves the time-delays between the emission of the two electrons for different energy sharings.
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Transition metals with their densely confined and strongly coupled valence electrons are key constituents of many materials with unconventional properties, such as high-Tc superconductors, Mott insulators and transition-metal dichalcogenides. Strong electron interaction offers a fast and efficient lever to manipulate their properties with light, creating promising potential for next-generation electronics. However, the underlying dynamics is a fast and intricate interplay of polarization and screening effects, which is poorly understood. It is hidden below the femtosecond timescale of electronic thermalization, which follows the light-induced excitation. Here, we investigate the many-body electron dynamics in transition metals before thermalization sets in. We combine the sensitivity of intra-shell transitions to screening effects with attosecond time resolution to uncover the interplay of photo-absorption and screening. First-principles time-dependent calculations allow us to assign our experimental observations to ultrafast electronic localization on d-orbitals. The latter modifies the whole electronic structure as well as the collective dynamic response of the system on a timescale much faster than the light-field cycle. Our results demonstrate a possibility for steering the electronic properties of solids prior to electron thermalization, suggesting that the ultimate speed of electronic phase transitions is limited only by the duration of the controlling laser pulse. Furthermore, external control of the local electronic density serves as a fine tool for testing state-of-the art models of electron-electron interactions. We anticipate our study to facilitate further investigations of electronic phase transitions, laser-metal interactions and photo-absorption in correlated electron systems on its natural timescale.
Up to this point streak-cameras have been a powerful tool for temporal characterization of ultrafast light pulses even at the single photon level. However, the low signal-to-noise ratio in the infrared range prevents measurement on weak light sources in the telecom regime. We present an approach to circumvent this problem. The method utilizes an up-conversion process in periodically poled waveguides in Lithium Niobate. We convert single photons from a parametric down-conversion source in order to reach the point of maximum detection efficiency of commercially available streak-cameras. We explore phase-matching configurations to investigate the up-conversion scheme in real-world applications.
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