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Register a new usermuSR in Ce_{1-x}La_xAl_3: anisotropic Kondo effect?
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Added by
Douglas E. MacLaughlin
Publication date
2002
fields
Physics
and research's language is
English
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Zero-field muSR experiments in the heavy-fermion alloys Ce_{1-x}La_xAl_3, x = 0 and 0.2, examine a recent proposal that the system exhibits a strong anisotropic Kondo effect. We resolve a damped oscillatory component for both La concentrations, indicative of disordered antiferromagnetism. For x = 0.2 the oscillation frequency decreases smoothly with increasing temperature, and vanishes at the specific heat anomaly temperature T* approx 2.2 K. Our results are consistent with the view that T* is due to a magnetic transition rather than anisotropic Kondo behavior.
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We study the evolution of the Kondo effect in heavy fermion compounds, Yb(Fe$_{1-x}$Co$_{x}$)$_{2}$Zn$_{20}$ (0$leqslant$ x $leqslant$ 1), by means of temperature-dependent electric resistivity and specific heat. The ground state of YbFe$_2$Zn$_{20}$ can be well described by a Kondo model with degeneracy $N$ = 8 and a $T_Ksim$30 K. In the presence of a very similar total CEF splitting with YbFe$_2$Zn$_{20}$, the ground state of YbCo$_2$Zn$_{20}$ is close to a Kondo state with degeneracy $N$ = 2 and a much lower $T_Ksim$ 2 K. Upon Co substitution, the coherence temperature of YbFe$_2$Zn$_{20}$ is suppressed, accompanied by an emerging Schottky-like feature in specific heat associated with the thermal depopulation of CEF levels upon cooling. For 0.4$lesssim$ x $lesssim$ 0.9, the ground state remains roughly the same which can be qualitatively understood by Kondo effect in the presence of CEF splitting. There is no clear indication of Kondo coherence observable in resistivity within this substitution range down to 500 mK. The coherence re-appears at around x$gtrsim$ 0.9 and the coherence temperature increases with higher Co concentration levels.
The specific heat C of Ce_{0.8}La_{0.2}Al_{3} has been measured as a function of temperature T in magnetic fields up to 14 T. A large peak in C at 2.3 K has recently been ascribed to an anisotropic Kondo effect in this compound. A 14-T field depresses the temperature of the peak by only 0.2 K, but strongly reduces its height. The corresponding peak in C/T shifts from 2.1 K at zero field to 1.7 K at 14 T. The extrapolated specific heat coefficient C/T(T->0) increases with field over the range studied. We show that these trends are inconsistent with the anisotropic Kondo model.
The failed Kondo insulator CeNiSn has long been suspected to be a nodal metal, with a node in the hybridization matrix elements. Here we carry out a series of Nernst effect experiments to delineate whether the severely anisotropic magnetotransport coefficients do indeed derive from a nodal metal or can simply be explained by a highly anisotropic Fermi surface. Our experiments reveal that despite an almost 20-fold anisotropy in the Hall conductivity, the large Nernst signal is isotropic. Taken in conjunction with the magnetotransport anisotropy, these results provide strong support for an isotropic Fermi surface with a large anisotropy in quasiparticle mass derived from a nodal hybridization.
We report measurements of the thermoelectric power (TEP) for a series of Pb(1-x)Tl(x)Te crystals with x = 0.0 to 1.3%. Although the TEP is very large for x = 0.0, using a single band analysis based on older work for dilute magnetic alloys we do find evidence for a Kondo contribution of 11 - 18 uV/K. This analysis suggests that Tk is ~ 50 - 70 K, a factor 10 higher than previously thought.
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