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Register a new userImpurity Moments Conceal Low-Energy Relaxation of Quantum Spin Liquids
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We scrutinize the magnetic properties of $kappa$-(BEDT-TTF)$_2$Hg(SCN)$_2$Cl through its first-order metal-insulator transition at $T_{rm CO}=30$ K by means of $^1$H nuclear magnetic resonance (NMR). While in the metal we find Fermi-liquid behavior with temperature-independent $(T_1T)^{-1}$, the relaxation rate exhibits a pronounced enhancement when charge order sets in. The NMR spectra remain unchanged through the transition and no magnetic order stabilizes down to 25 mK. Similar to the isostructural spin-liquid candidates $kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$ and $kappa$-(BEDT-TTF)$_2$Ag$_2$(CN)$_3$, $T_1^{-1}$ acquires a dominant maximum (here around 5 K). Field-dependent experiments identify the low-temperature feature as a dynamic inhomogeneity contribution that is typically dominant over the intrinsic relaxation but gets suppressed with magnetic field.
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The electrodynamic response of organic spin liquids with highly-frustrated triangular lattices has been measured in a wide energy range. While the overall optical spectra of these Mott insulators are governed by transitions between the Hubbard bands, distinct in-gap excitations can be identified at low temperatures and frequencies which we attribute to the quantum spin liquid state. For the strongly correlated $beta^{prime}$-EtMe$_3$-Sb-[Pd(dmit)$_2$]$_2$, we discover enhanced conductivity below $175~{rm cm}^{-1}$, comparable to the energy of the magnetic coupling $Japprox 250$ K. For $omegarightarrow 0$ these low-frequency excitations vanish faster than the charge-carrier response subject to Mott-Hubbard correlations, resulting in a dome-shape band peaked at 100~cm. Possible relations to spinons, magnons and disorder are discussed.
Quantum spin-liquids are strongly correlated phases of matter displaying a highly entangled ground state. Due to their unconventional nature, finding experimental signatures of these states has proven to be a remarkable challenge. Here we show that the effects of local impurities can provide strong signatures of a Dirac quantum spin-liquid state. Focusing on a gapless Dirac quantum spin-liquid state as realized in NaYbO$_2$, we show that single magnetic impurity coupled to the quantum spin-liquid state creates a resonant spinon peak at zero frequency, coexisting the original Dirac spinons. We explore the spatial dependence of this zero-bias resonance, and show how different zero modes stemming from several impurities interfere. We finally address how such spinon zero-mode resonances can be experimentally probed with inelastic spectroscopy and electrically-driven paramagnetic resonance with scanning tunnel microscopy. Our results put forward impurity engineering as a means of identifying Dirac quantum spin-liquids with scanning probe techniques, highlighting the dramatic impact of magnetic impurities in a macroscopically entangled many-body ground state.
Spin liquids are quantum phases of matter that exhibit a variety of novel features associated with their topological character. These include various forms of fractionalization - elementary excitations that behave as fractions of an electron. While there is not yet entirely convincing experimental evidence that any particular material has a spin liquid ground state, in the past few years, increasing evidence has accumulated for a number of materials suggesting that they have characteristics strongly reminiscent of those expected for a quantum spin liquid.
We consider zero temperature behavior of dynamic response functions of 1D systems near edges of support in momentum-energy plane $(k, omega).$ The description of the singularities of dynamic response functions near an edge $epsilon(k)$ is given by the effective Hamiltonian of a mobile impurity moving in a Luttinger liquid. For Galilean-invariant systems, we relate the parameters of such an effective Hamiltonian to the properties of the function $epsilon (k).$ This allows us to express the exponents which characterize singular response functions of spinless bosonic or fermionic liquids in terms of $epsilon(k)$ and Luttinger liquid parameters for any $k.$ For an antiferromagnetic Heisenberg spin-1/2 chain in a zero magnetic field, SU(2) invariance fixes the exponents from purely phenomenological considerations.
Quantum spin liquids attract great interest due to their exceptional magnetic properties characterized by the absence of long-range order down to low temperatures despite the strong magnetic interaction. Commonly, these compounds are strongly correlated electron systems, and their electrodynamic response is governed by the Mott gap in the excitation spectrum. Here we summarize and discuss the optical properties of several two-dimensional quantum spin liquid candidates. First we consider the inorganic material Herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$ and related compounds, which crystallize in a kagome lattice. Then we turn to the organic compounds $beta^{prime}$-EtMe$_3$-Sb-[Pd(dmit)$_2$]$_2$, $kappa$-(BEDT-TTF)$_2$Ag$_2$(CN)$_3$ and $kappa$-(BEDT-TTF)$_2$Cu$_2$(CN)$_3$, where the spins are arranged in an almost perfect triangular lattice, leading to strong frustration. Due to differences in bandwidth, the effective correlation strength varies over a wide range, leading to a rather distinct behavior as far as the electrodynamic properties are concerned. We discuss the spinon contributions to the optical conductivity in comparison to metallic quantum fluctuations in the vicinity of the Mott transition.
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