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Register a new userObservation of superconductivity in pressurized Weyl semimetal candidate TaIrTe4
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Here we report the observation of superconductivity in pressurized type-II Weyl semimetal (WSM) candidate TaIrTe4 by means of complementary high-pressure transport and synchrotron X-ray diffraction measurements. We find that TaIrTe4 shows superconductivity with transition temperature (TC) of 0.57 K at the pressure of ~23.8 GPa. Then, the TC value increases with pressure and reaches ~2.1 K at 65.7 GPa. In situ high-pressure Hall coefficient (RH) measurements at low temperatures demonstrate that the positive RH increases with pressure until the critical pressure of the superconducting transition is reached, but starts to decrease upon further increasing pressure. Above the critical pressure, the positive magnetoresistance effect disappears simultaneously. Our high pressure X-ray diffraction measurements reveal that, at around the critical pressure the lattice of the TaIrTe4 sample is distorted by the application of pressure and its volume is reduced by ~19.2%, the value of which is predicted to result in the change of the electronic structure significantly. We propose that the pressure-induced distortion in TaIrTe4 is responsible for the change of topology of Fermi surface and such a change favors the emergence of superconductivity. Our results clearly demonstrate the correlation among the lattice distortion, topological physics and superconductivity in the WSM.
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The search for unconventional superconductivity in Weyl semimetal materials is currently an exciting pursuit, since such superconducting phases could potentially be topologically nontrivial and host exotic Majorana modes. The layered material TaIrTe4 is a newly predicted time-reversal invariant type II Weyl semimetal with minimum number of Weyl points. Here, we report the discovery of surface superconductivity in Weyl semimetal TaIrTe4. Our scanning tunneling microscopy/spectroscopy (STM/S) visualizes Fermi arc surface states of TaIrTe4 that are consistent with the previous angle-resolved photoemission spectroscopy (ARPES) results. By a systematic study based on STS at ultralow temperature, we observe uniform superconducting gaps on the sample surface. The superconductivity is further confirmed by electrical transport measurements at ultralow temperature, with an onset transition temperature (Tc) up to 1.54 K being observed. The normalized upper critical field h*(T/Tc) behavior and the stability of the superconductivity against the ferromagnet indicate that the discovered superconductivity is unconventional with the p-wave pairing. The systematic STS, thickness and angular dependent transport measurements reveal that the detected superconductivity is quasi-one-dimensional (quasi-1D) and occurs in the surface states. The discovery of the surface superconductivity in TaIrTe4 provides a new novel platform to explore topological superconductivity and Majorana modes.
Two-dimensional (2D) transition-metal dichalcogenide (TMDs) MoTe2 has attracted much attention due to its predicted Weyl semimetal (WSM) state and a quantum spin Hall insulator in bulk and monolayer form, respectively. We find that the superconductivity in MoTe2 single crystal can be much enhanced by the partial substitution of the Te ions by the S ones. The maximum of the superconducting temperature TC of MoTe1.8S0.2 single crystal is about 1.3 K. Compared with the parent MoTe2 single crystal (TC=0.1 K), nearly 13-fold in TC is improved in MoTe1.8S0.2 one. The superconductivity has been investigated by the resistivity and magnetization measurements. MoTe2-xSx single crystals belong to weak coupling superconductors and the improvement of the superconductivity may be related to the enhanced electron-phonon coupling induced by the S-ion substitution. A dome-shape superconducting phase diagram is obtained in the S-doped MoTe2 single crystals. MoTe2-xSx materials may provide a new platform for our understanding of superconductivity phenomena and topological physics in TMDs.
Here we report the observation of pressure-induced superconductivity in type-II Weyl semimetal (WSM) candidate NbIrTe4 and the evolution of its Hall coefficient (RH), magnetoresistance (MR), and lattice with increasing pressure to ~57 GPa. These results provide a significant opportunity to investigate the universal high-pressure behavior of ternary WSMs, including the sister compound TaIrTe4 that has been known through our previous studies. We find that the pressure-tuned evolution from the WSM to the superconducting (SC) state in these two compounds exhibit the same trend, i.e., a pressure-induced SC state emerges from the matrix of the non-superconducting WSM state at ~ 27 GPa, and then the WSM state and the SC state coexist up to 40 GPa. Above this pressure, an identical high-pressure behavior, characterized by almost the same value of RH and MR in its normal state and the same value of Tc in its SC state, appears in both compounds. Our results not only reveal a universal connection between the WSM state and SC state, but also demonstrate that NbIrTe4 and TaIrTe4 can make the same contribution to the normal and SC states that inhabit in the high-pressure phase, although these two compounds have dramatically different topological band structure at ambient pressure.
The relation between the polar structural instability and superconductivity in a Weyl semimetal candidate MoTe2 has been clarified by finely controlled physical and chemical pressure. The physical pressure as well as the chemical pressure, i.e., the Se substitution for Te, enhances the superconducting transition temperature Tc at around the critical pressure where the polar structure transition disappears. From the heat capacity and thermopower measurements, we ascribe the significant enhancement of Tc at the critical pressure to a subtle modification of the phonon dispersion or the semimetallic band structure upon the polar-to-nonpolar transition. On the other hand, the physical pressure, which strongly reduces the interlayer distance, is more effective on the suppression of the polar structural transition and the enhancement of Tc as compared with the chemical pressure, which emphasizes the importance of the interlayer coupling on the structural and superconducting instability in MoTe2.
The layered ternary compound TaIrTe4 is an important candidate to host the recently predicted type-II Weyl Fermions. However, a direct and definitive proof of the absence of inversion symmetry in this material, a prerequisite for the existence of Weyl Fermions, has so far remained evasive. Herein, an unambiguous identification of the broken inversion symmetry in TaIrTe4 is established using angle-resolved polarized Raman spectroscopy. Combining with high-resolution transmission electron microscopy, we demonstrate an efficient and nondestructive recipe to determine the exact crystallographic orientation of TaIrTe4 crystals. Such technique could be extended to the fast identification and characterization of other type-II Weyl Fermions candidates. A surprisingly strong in-plane electrical anisotropy in TaIrTe4 thin flakes is also revealed, up to 200% at 10K, which is the strongest known electrical anisotropy for materials with comparable carrier density, notably in such good metals as copper and silver.
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