No Arabic abstract
Correlation effects in CuO$_2$ layers give rise to a complicated landscape of collective excitations in high-T$_{rm c}$ cuprates. Their description requires an accurate account for electronic fluctuations at a very broad energy range and remains a challenge for the theory. Particularly, there is no conventional explanation of the experimentally observed `resonant antiferromagnetic mode, which is often considered to be a mediator of superconductivity. Here we model spin excitations of the hole-doped cuprates in the paramagnetic regime and show that this antiferromagnetic mode is associated with electronic transitions between anti-nodal X and Y points of the quasiparticle band that is pinned to the Fermi level. We observe that upon doping of 7-12% the electronic spectral weight redistribution leads to the formation of a very stable quasiparticle dispersion due to strong correlation effects. The reconstruction of the Fermi surface results in a flattening of the quasiparticle band at the vicinity of the nodal ${rm M}Gamma/2$ point, accompanied by a high density of charge carriers. Collective excitations of electrons between the nodal ${rm M}Gamma/2$ and ${rm XM}/2$ points form the additional magnetic holes state in magnetic spectrum, which protects the antiferromagnetic fluctuation. Further investigation of the evolution of spin fluctuations with the temperature and doping allowed us to observe the incipience of the antiferromagnetic ordering already in the paramagnetic regime above the transition temperature. Additionally, apart from the most intensive low-energy magnetic excitations, the magnetic spectrum reveals less intensive collective spin fluctuations that correspond to electronic processes between peaks of the single-particle spectral function.
We study the electronic structure of the ladder compounds (SrCa)CuO 14-24-41 and SrCuO 123. LDA calculations for both give similar Cu 3d-bands near the Fermi energy. The hopping parameters estimated by fitting LDA energy bands show a strong anisotropy between the t_perp t_par intra-ladder hopping and small inter-ladder hopping. A downfolding method shows that this anisotropy arises from the ladder structure.The conductivity perpendicular to the ladders is computed assuming incoherent tunneling giving a value close to experiment.
Magnetic structures of organic Mott insulators X[Pd(dmit)2]2 (X=Me4P, Me4Sb), of which electronic states are located near quantum spin liquid (X=EtMe3Sb), are demonstrated by 13C NMR. Antiferromagnetic spectra and nuclear relaxations show two distinct magnetic moments within each Pd(dmit)2 molecule, which cannot be described by single band dimer-Mott model and requires intramolecular electronic correlation. This unconventional fragmentation of S = 1/2 electron spin with strong quantum fluctuation is presumably caused by nearly degenerated intramolecular multiple orbitals, and shares a notion of quantum liquids where electronic excitations are fractionalized and S = 1/2 spin is no longer an elementary particle.
Unconventional symmetry-breaking phenomena due to nontrivial order parameters attract increasing attention in strongly correlated electron systems. Here, we predict theoretically the occurrence of nanoscale spontaneous spin-current, called the spin loop-current (sLC) order, as a promising origin of the pseudogap and electronic nematicity in cuprates. We reveal that the sLC is driven by the odd-parity electron-hole condensation that are mediated by transverse spin fluctuations around the pseudogap temperature $T^*$. At the same temperature, odd-parity magnon pair condensation occurs. The sLC order is hidden in that neither internal magnetic field nor charge density modulation is induced, whereas the predicted sLC with finite wavenumber naturally gives the Fermi arc structure. In addition, the fluctuations of sLC order work as attractive pairing interaction between adjacent hot spots, which enlarges the d-wave superconducting transition temperature $T_c$. The sLC state will be a key ingredient in understanding the pseudogap, electronic nematicity as well as superconductivity in cuprates and other strongly correlated metals.
The electronic structure of a new charge-density-wave/ superconductor system, 1T-CuxTiSe2, has been studied by photoemission spectroscopy. A correlated semiconductor band structure is revealed for the undoped case. With Cu doping, the charge density wave is suppressed by the raising of the chemical potential, while the superconductivity is enhanced by the enhancement of the density of states. Moreover, the strong scattering at high doping might be responsible for the suppression of superconductivity in that regime.
Among heavy-fermion metals, Ce$_3$Pd$_{20}$Si$_6$ is one of the heaviest-electron systems known to date. Here we used high-resolution neutron spectroscopy to observe low-energy magnetic scattering from a single crystal of this compound in the paramagnetic state. We investigated its temperature dependence and distribution in momentum space, which was not accessible in earlier measurements on polycrystalline samples. At low temperatures, a quasielastic magnetic response with a half-width {Gamma}=0.1 meV persists with varying intensity all over the Brillouin zone. It forms a broad hump centered at the (111) scattering vector, surrounded by minima of intensity at (002), (220) and equivalent wave vectors. The momentum-space structure distinguishes this signal from a simple crystal-field excitation at 0.31 meV, suggested previously, and rather lets us ascribe it to short-range dynamical correlations between the neighboring Ce ions, mediated by the itinerant heavy f-electrons via the RKKY mechanism. With increasing temperature, the energy width of the signal follows the conventional T$scriptstyle^{1/2}$ law, {Gamma}(T) = {Gamma}$_0$ + A*T$scriptstyle^{1/2}$. The momentum-space symmetry of the quasielastic response suggests that it stems from the simple-cubic Ce sublattice occupying the 8c Wyckoff site, whereas the crystallographically inequivalent 4a site remains magnetically silent in this material.