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Excitation function of the alpha particle induced nuclear reactions on enriched $^{116}$Cd, production of the theranostic isotope $^{117m}$Sn

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 Added by Ferenc Ditr\\'oi Dr
 Publication date 2016
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and research's language is English




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$^{117m}$Sn is one of the radioisotopes can be beneficially produced through alpha particle irradiation. The targets were prepared by deposition of $^{116}$Cd metal onto high purity 12 $mu$m thick Cu backing. The average deposited thickness was 21.9 $mu$m. The beam energy was thoroughly measured by Time of Flight (TOF) methods and proved to be 51.2 MeV. For the experiment the well-established stacked foil technique was used. In addition to the Cd targets, Ti foils were also inserted into the stacks for energy and intensity monitoring. The Cu backings were also used for monitoring and as recoil catcher of the reaction products from the cadmium layer. The activities of the irradiated foils were measured with HPGe detector for gamma-ray spectrometry and cross section values were determined. As a result excitation functions for the formation of $^{117m}$Sn, $^{117m,g}$In, $^{116m}$In, $^{115m}$In and $^{115m,g}$Cd from enriched $^{116}$Cd were deduced and compared with the available literature data and with the results of the nuclear reaction model code calculations EMPIRE 3.2 and TALYS 1.8. Yield curves were also deduced for the measured nuclear reactions and compared with the literature.



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Double beta decay of $^{116}$Cd has been investigated with the help of radiopure enriched $^{116}$CdWO$_4$ crystal scintillators in the experiment Aurora. The half-life of $^{116}$Cd relatively to the 2$ u$2$beta$ decay of $^{116}$Cd to the ground level of $^{116}$Sn is measured with the highest up-to-date accuracy as $T_{1/2}$ = [2.69 $pm$ 0.02 (stat.) $pm$ 0.14 (syst.)] $times$ 10$^{19}$ yr. A new improved limit on the 0$ u$2$beta$ decay of $^{116}$Cd to the ground state of $^{116}$Sn is set as $T_{1/2}geq 2.4 times 10^{23}$ yr at 90% C.L., that corresponds to the effective Majorana neutrino mass limit in the range $langle$$m_ u$$rangle$ $le$ $(1.1-1.6)$ eV, depending on the nuclear matrix elements used in the estimations. New improved limits on other $2beta$ processes in $^{116}$Cd (decays with majoron emission, transitions to excited levels of $^{116}$Sn) were set at the level of $T_{1/2}geq 10^{21}-10^{22}$ yr.
In the frame of a systematic study of charged particle production routes of medically relevant radionuclei, the excitation function for indirect production of $^{178m}$Ta through $^{nat}$Hf($alpha$,xn)$^{178}$W-$^{178m}$Ta nuclear reaction was measured for the first time up to 40 MeV. In parallel, the side reactions $^{nat}$Hf($alpha$,x)$^{179,177,176,175}$W, $^{183,182,178g,177,176,175}$Ta, $^{179m,177m,175}$Hf were also assessed. Stacked foil irradiation technique and $gamma$-ray spectrometry were used. New experimental cross section data for the $^{nat}$Ta(d,xn)$^{178}$W reaction are also reported up to 40 MeV. The measured excitation functions are compared with the results of the ALICE-IPPE, and EMPIRE nuclear reaction model codes and with the TALYS 1.4 based data in the TENDL-2013 library. The thick target yields were deduced and compared with yields of other charged particle ((p,4n), (d,5n) and ($^3$He,x)) production routes for $^{178}$W.
One of the few p nuclei with an odd number of protons is 113In. Reaction cross sections of 113In(alpha,gamma)117Sb and 113In(alpha,n)116Sb have been measured with the activation method at center-of-mass energies between 8.66 and 13.64 MeV, close to the astrophysically relevant energy range. The experiments were carried out at the cyclotron accelerator of ATOMKI. The activities were determined by off-line detection of the decay gamma rays with a HPGe detector. Measured cross sections and astrophysical S factor results are presented and compared with statistical model calculations using three different alpha+nucleus potentials. The comparison indicates that the standard rates used in the majority of network calculations for these reactions were too fast due to the energy dependence of the optical alpha potential at low energy.
130 - M. Debowski 1997
Double differential cross sections have been measured for pi+ and K+ emitted around midraidity in d+A and He+A collisions at a beam kinetic energy of 1.15 GeV/nucleon. The total pi+ yield increases by a factor of about 2 when using an alpha projectile instead of a deuteron whereas the K+ yield increases by a factor of about 4. According to transport calculations, the K+ enhancement depends both on the number of hadron-hadron collisions and on the energy available in those collisions: their center-of-mass energy increases with increasing number of projectile nucleons.
The double-beta decay of $^{116}$Cd has been investigated with the help of radiopure enriched $^{116}$CdWO$_4$ crystal scintillators (mass of 1.162 kg) at the Gran Sasso underground laboratory. The half-life of $^{116}$Cd relatively to the $2 u2beta$ decay to the ground state of $^{116}$Sn was measured with the highest up-to-date accuracy as $T_{1/2}=(2.63^{+0.11}_{-0.12})times10^{19}$ yr. A new improved limit on the 0$ u$2$beta$ decay of $^{116}$Cd to the ground state of $^{116}$Sn was set as $T_{1/2}geq 2.2 times 10^{23}$ yr at 90% C.L., which is the most stringent known restriction for this isotope. It corresponds to the effective Majorana neutrino mass limit in the range $langle m_ uranglele(1.0-1.7)$ eV, depending on the nuclear matrix elements used in the estimations. New improved half-life limits for the 0$ u$2$beta$ decay with majoron(s) emission, Lorentz-violating $2 u2beta$ decay and $2beta$ transitions to excited states of $^{116}$Sn were set at the level of $T_{1/2}geq 10^{20}-10^{22}$ yr. New limits for the hypothetical lepton-number violating parameters (right-handed currents admixtures in weak interaction, the effective majoron-neutrino coupling constants, R-parity violating parameter, Lorentz-violating parameter, heavy neutrino mass) were set.
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