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Register a new userRoom-temperature transport properties of spin-orbit coupled Fermi systems: Spin thermoelectric effects, phonon skew scattering
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In this note we summarize our recent results for the temperature dependence of transport coefficients of metallic films in the presence of spin-orbit coupling. Our focus is on (i) the spin Nernst and the thermal Edelstein effects, and (ii) the phonon skew scattering contribution to the spin Hall conductivity, which is relevant for the temperature dependence of the spin Hall angle. Depending on the parameters, the latter is expected to show a non-monotonous behavior.
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We study the effects caused by Rashba and Dresselhaus spin-orbit coupling over the thermoelectric transport properties of a single-electron transistor, viz., a quantum dot connected to one-dimensional leads. Using linear response theory and employing the numerical renormalization group method, we calculate the thermopower, electrical and thermal conductances, dimensionless thermoelectric figure of merit, and study the Wiedemann-Franz law, showing their temperature maps. Our results for all those properties indicate that spin-orbit coupling drives the system into the Kondo regime. We show that the thermoelectric transport properties, in the presence of spin-orbit coupling, obey the expected universality of the Kondo strong coupling fixed point. In addition, our results show a notable increase in the thermoelectric figure of merit, caused by the spin-orbit coupling in the one-dimensional quantum dot leads.
We present a detailed analysis of the skew-scattering contribution to the spin Hall conductivity using an extended version of the resonant scattering model of Fert and Levy [Phys. Rev. Lett. {bf 106}, 157208 (2011)]. For $5d$ impurities in a Cu host, the proposed phase shift model reproduces the corresponding first-principles calculations. Crucial for that agreement is the consideration of two scattering channels related to $p$ and $d$ impurity states, since the discussed mechanism is governed by a subtle interplay between the spin-orbit and potential scattering in both angular-momentum channels. It is shown that the potential scattering strength plays a decisive role for the magnitude of the spin Hall conductivity.
We study theoretically some symmetry properties of spin currents and spin polarizations in multi-terminal mesoscopic spin-orbit coupled systems. Based on a scattering wave function approach, we show rigorously that in the equilibrium state no finite spin polarizations can exist in a multi-terminal mesoscopic spin-orbit coupled system (both in the leads and in the spin-orbit coupled region) and also no finite equilibrium terminal spin currents can exist. By use of a typical two-terminal mesoscopic spin-orbit coupled system as the example, we show explicitly that the nonequilibrium terminal spin currents in a multi-terminal mesoscopic spin-orbit coupled system are non-conservative in general. This non-conservation of terminal spin currents is not caused by the use of an improper definition of spin current but is intrinsic to spin-dependent transports in mesoscopic spin-orbit coupled systems. We also show that the nonequilibrium lateral edge spin accumulation induced by a longitudinal charge current in a thin strip of textit{finite} length of a two-dimensional electronic system with intrinsic spin-orbit coupling may be non-antisymmetric in general, which implies that some cautions may need to be taken when attributing the occurrence of nonequilibrium lateral edge spin accumulation induced by a longitudinal charge current in such a system to an intrinsic spin Hall effect.
We measure and analyze the effective spin Hall angle of platinum in the low residual resistivity regime by second harmonic measurements of the spin-orbit torques for a multilayer of Pt/Co/AlO$_x$. An angular dependent study of the torques allows us to extract the effective spin Hall angle responsible for the damping-like torque in the system. We observe a strikingly non-monotonic and reproducible temperature dependence of the torques. This behavior is compatible with recent theoretical predictions which include both intrinsic and extrinsic (impurities and phonons) contributions to the spin Hall effect at finite temperature.
The ultimate goal of spintronics is achieving electrically controlled coherent manipulation of the electron spin at room temperature to enable devices such as spin field-effect transistors. With conventional materials, coherent spin precession has been observed in the ballistic regime and at low temperatures only. However, the strong spin anisotropy and the valley character of the electronic states in 2D materials provide unique control knobs to manipulate spin precession. Here, by manipulating the anisotropic spin-orbit coupling in bilayer graphene by the proximity effect to WSe$_2$, we achieve coherent spin precession in the absence of an external magnetic field, even in the diffusive regime. Remarkably, the sign of the precessing spin polarization can be tuned by a back gate voltage and by a drift current. Our realization of a spin field-effect transistor at room temperature is a cornerstone for the implementation of energy-efficient spin-based logic.
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