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Register a new userRemote creation of strong and coherent emissions in air with two-color ultrafast laser pulses
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We experimentally demonstrate generation of strong narrow-bandwidth emissions with excellent coherent properties at ~391 nm and ~428 nm from molecular ions of nitrogen inside a femtosecond filament in air by an orthogonally polarized two-color driver field (i. e., 800 nm laser pulse and its second harmonic). The durations of the coherent emissions at 391 nm and 428 nm are measured to be ~2.4 ps and ~7.8 ps respectively, both of which are much longer than the duration of the pump and its second harmonic pulses. Furthermore, the measured temporal decay characteristics of the excited molecular systems suggest an instantaneous population inversion mechanism that may be achieved in molecular nitrogen ions at an ultrafast time scale comparable to the 800 nm pump pulse.
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We investigate the generation of broadband terahertz (THz) pulses with phase singularity from air plasmas created by fundamental and second harmonic laser pulses. We show that when the second harmonic beam carries a vortex charge, the THz beam acquires a vortex structure as well. A generic feature of such THz vortex is that the intensity is modulated along the azimuthal angle, which can be attributed to the spatially varying relative phase difference between the two pump harmonics. Fully space and time resolved numerical simulations reveal that transverse instabilities of the pump further affect the emitted THz field along nonlinear propagation, which produces additional singularities resulting in a rich vortex structure. The predicted intensity modulation is experimentally demonstrated with a thermal camera, in excellent agreement with simulation results. The presence of phase singularities in the experiment is revealed by astigmatic transformation of the beam using a cylindrical mirror.
We experimentally investigate generation of molecular nitrogen-ion lasers with two femtosecond laser pulses at different wavelengths. The first pulse serves as the pump which ionizes the nitrogen molecules and excites the molecular ions to excited electronic states. The second pulse serves as the probe which leads to stimulated emission from the excited molecular ions. We observe that changing the angle between the polarization directions of the two pulses gives rise to elliptically polarized molecular nitrogen-ion laser fields, which is interpreted as a result of strong birefringence of the gain medium near the wavelengths of the molecular nitrogen-ion laser.
Ultrashort long-wave infrared (LWIR) laser pulses can resonantly excite vibrations in N2 and O2 through a two-photon transition. The absorptive, vibrational component of the ultrafast optical nonlinearity grows in time, starting smaller than, but quickly surpassing, the electronic, rotational, and vibrational refractive components. The growth of the vibrational component results in a novel mechanism of 3rd harmonic generation, providing an additional two-photon excitation channel, fundamental + 3rd harmonic. The original and emergent two-photon excitations drive the resonance exactly out of phase, causing spatial decay of the absorptive, vibrational nonlinearity. This nearly eliminates two-photon vibrational absorption. Here we present simulations and analytical calculations demonstrating how these processes modify the ultrafast optical nonlinearity in air. The results reveal nonlinear optical phenomena unique to the LWIR regime of ultrashort pulse propagation in atmosphere.
We experimentally demonstrate energy exchange between a delay-tuned femtosecond beam and two delay-fixed ones as they spatiotemporally overlapped and experienced filamentation in air. The energy exchange process in the relative time delay is dramatically elongated up to 40 ps in the presence of plasma grating, indicating that filamentary beams coupling may be an effective method for filament control.
We study the propagation of 0.05-1 TW power, ultrafast laser pulses in a 10 meter long rubidium vapor cell. The central wavelength of the laser is resonant with the $D_2$ line of rubidium and the peak intensity in the $10^{12}-10^{14} ~W/cm^2$ range, enough to create a plasma channel with single electron ionization. We observe the absorption of the laser pulse for low energy, a regime of transverse confinement of the laser beam by the strong resonant nonlinearity for higher energies and the transverse broadening of the output beam when the nonlinearity is saturated due to full medium ionization. We compare experimental observations of transmitted pulse energy and transverse fluence profile with the results of computer simulations modeling pulse propagation. We find a qualitative agreement between theory and experiment that corroborates the validity of our propagation model. While the quantitative differences are substantial, the results show that the model can be used to interpret the observed phenomena in terms of self-focusing and channeling of the laser pulses by the saturable nonlinearity and the transparency of the fully ionized medium along the propagation axis.
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