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Register a new userAnion height dependence of Tc for the Fe-based superconductor
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Yoshikazu Mizuguchi
Publication date
2010
fields
Physics
and research's language is
English
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We have established a plot of the anion height dependence of Tc for the typical Fe-based superconductors. The plot appeared a symmetric curve with a peak around 1.38 A. Both data at ambient pressure and under high pressure obeyed the unique curve. This plot will be one of the key strategies for both understanding the mechanism of Fe-based superconductivity and search for the new Fe-based superconductors with higher Tc.
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In this study, we performed high-pressure electrical resistivity measurements of polycrystalline FeSe in the pressure range of 1-16.0 GPa at temperatures of 4-300 K. A precise evaluation of Tc from zero-resistivity temperatures revealed that Tc shows a slightly distorted dome-shaped curve, with maximum Tc (30 K) at 6 GPa, which is lower than a previously reported Tc value (~37 K). With the application of pressure, the temperature dependence of resistivity above Tc changes dramatically to a linear dependence; a non-Fermi-liquid-like high-Tc phase appears above 3 GPa. We found a striking correlation between Tc and the Se height: the lower the Se height, the more enhanced is Tc. Moreover, this relation is broadly applicable to other iron pnictides, strongly indicating that high-temperature superconductivity can appear only around the optimum anion height (~1.38A). On the basis of these results, we suggest that the anion height should be considered as a key determining factor of Tc of iron-based superconductors containing various anions.
We investigate the importance of superconducting order parameter fluctuations in the 122 family of Fe-based superconductors, using high-resolution specific heat and thermal expansion data of various Ba$_{1-x}$K$_x$Fe$_2$As$_2$ single crystals covering a large range of the phase diagram from the strongly underdoped to the overdoped regime. By applying scaling relations of the 3d-XY and the 3d-Lowest-Landau-Level (3d-LLL) fluctuation models to data measured in different magnetic fields, we demonstrate that a strong increase of the critical fluctuation regime is responsible for the transition broadening in magnetic fields, which is a direct consequence of a magnetic-field-induced finite size effect due to a reduction of the effective dimensionality by a decreasing magnetic length scale related to the mean vortex separation and the confinement of quasiparticles in low Landau levels. The fluctuations are stronger in the underdoped and overdoped regimes and appear to be weakest at optimal doping.
Pinning force data, Fp, of a variety of Fe-based high-Tc superconductors (11-, 111-, 122- and 1111-type) were analyzed by means of a scaling approach based on own experimental data and an extensive collection of literature data. The literature data were mostly replotted, but also converted from critical current measurements together with data for the irreversibility line when available from the same authors. Using the scaling approaches of Dew-Hughes and Kramer, we determined the scaling behavior and the best fits to the theory. The data of most experiments analyzed show a good scaling behavior at high temperatures when plotting the normalized pinning force Fp/Fp,max versus the irreversibility field, Hirr. The resulting peak positions, h0, were found at 0.3 for the 11-type materials, at 0.48 for the 111-type materials, between 0.32 and 0.5 for the 1111-type materials and between 0.25 and 0.71 for the 122-type materials. This high peak position ensures a good performance of the materials in high applied magnetic fields and is, therefore, a very promising result concerning the possible applications of the Fe-based high-Tc superconductors.
Ultrahigh resolution angle-resolved photoemission spectroscopy with low-energy photons is used to study the detailed momentum dependence of the well-known nodal kink dispersion anomaly of Bi2Sr2CaCu2O8+{delta}. We find that the kinks location transitions smoothly from a maximum binding energy of about 65 meV at the node of the d-wave superconducting gap to 55 meV roughly one-third of the way to the antinode. Meanwhile, the self-energy spectrum corresponding to the kink dramatically sharpens and intensifies beyond a critical point in momentum space. We discuss the possible bosonic spectrum in energy and momentum space that can couple to the k-space dispersion of the electronic kinks.
We report a sudden reversal in the pressure dependence of Tc in the iron-based superconductor CsFe2As2, similar to that discovered recently in KFe2As2 [Tafti et al., Nat. Phys. 9, 349 (2013)]. As in KFe2As2, we observe no change in the Hall coefficient at the zero temperature limit, again ruling out a Lifshitz transition across the critical pressure Pc. We interpret the Tc reversal in the two materials as a phase transition from one pairing state to another, tuned by pressure, and investigate what parameters control this transition. Comparing samples of different residual resistivity, we find that a 6-fold increase in impurity scattering does not shift Pc. From a study of X-ray diffraction on KFe2As2 under pressure, we report the pressure dependence of lattice constants and As-Fe-As bond angle. The pressure dependence of these lattice parameters suggests that Pc should be significantly higher in CsFe2As2 than in KFe2As2, but we find on the contrary that Pc is lower in CsFe2As2. Resistivity measurements under pressure reveal a change of regime across Pc, suggesting a possible link between inelastic scattering and pairing symmetry.
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