This two-paper series addresses and fixes the long-standing gauge invariance problem of angular momentum in gauge theories. This QED part reveals: 1) The spin and orbital angular momenta of electrons and photons can all be consistently defined gauge invariantly. 2) These gauge-invariant quantities can be conveniently computed via the canonical, gauge-dependent operators (e.g, $psi ^dagger vec x timesfrac 1i vec abla psi$) in the Coulomb gauge, which is in fact what people (unconsciously) do in atomic physics. 3) The renowned formula $vec xtimes(vec Etimesvec B)$ is a wrong density for the electromagnetic angular momentum. The angular distribution of angular-momentum flow in polarized atomic radiation is properly described not by this formula, but by the gauge invariant quantities defined here. The QCD paper [arXiv:0907.1284] will give a non-trivial generalization to non-Abelian gauge theories, and discuss the connection to nucleon spin structure.
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