No Arabic abstract
The whispering gallery modes (WGMs) of quartz microspheres are investigated for the purpose of strong coupling between single photons and atoms in cavity quantum electrodynamics (cavity QED). Within our current understanding of the loss mechanisms of the WGMs, the saturation photon number, n, and critical atom number, N, cannot be minimized simultaneously, so that an optimal sphere size is taken to be the radius for which the geometric mean, (n x N)^(1/2), is minimized. While a general treatment is given for the dimensionless parameters used to characterize the atom-cavity system, detailed consideration is given to the D2 transition in atomic Cesium (852nm) using fused-silica microspheres, for which the maximum coupling coefficient g/(2*pi)=750MHz occurs for a sphere radius a=3.63microns corresponding to the minimum for n=6.06x10^(-6). By contrast, the minimum for N=9.00x10^(-6) occurs for a sphere radius of a=8.12microns, while the optimal sphere size for which (n x N)^(1/2) is minimized occurs at a=7.83microns. On an experimental front, we have fabricated fused-silica microspheres with radii a=10microns and consistently observed quality factors Q=0.8x10^(7). These results for the WGMs are compared with corresponding parameters achieved in Fabry-Perot cavities to demonstrate the significant potential of microspheres as a tool for cavity QED with strong coupling.
We present and analyze a method where parametric (two-photon) driving of a cavity is used to exponentially enhance the light-matter coupling in a generic cavity QED setup, with time-dependent control. Our method allows one to enhance weak-coupling systems, such that they enter the strong coupling regime (where the coupling exceeds dissipative rates) and even the ultra-strong coupling regime (where the coupling is comparable to the cavity frequency). As an example, we show how the scheme allows one to use a weak-coupling system to adiabatically prepare the highly entangled ground state of the ultra-strong coupling system. The resulting state could be used for remote entanglement applications.
Normal mode splitting is observed in a cavity QED system, in which nitrogen vacancy centers in diamond nanocrystals are coupled to whispering gallery modes in a silica microsphere. The composite nanocrystal-microsphere system takes advantage of the exceptional spin properties of nitrogen vacancy centers as well as the ultra high quality factor of silica microspheres. The observation of the normal mode splitting indicates that the dipole optical interaction between the relevant nitrogen vacancy center and whispering gallery mode has reached the strong coupling regime of cavity QED.
Hybrid quantum systems based on spin ensembles coupled to superconducting microwave cavities are promising candidates for robust experiments in cavity quantum electrodynamics (QED) and for future technologies employing quantum mechanical effects. Currently the main source of decoherence in these systems is inho- mogeneous spin broadening, which limits their performance for the coherent transfer and storage of quantum information. Here we study the dynamics of a superconducting cavity strongly coupled to an ensemble of nitrogen-vacancy centers in diamond. We experimentally observe for the first time, how decoherence induced by a non-Lorentzian spin distribution can be suppressed in the strong-coupling regime - a phenomenon known as cavity protection. To demonstrate the potential of this effect for coherent control schemes, we show how appropriately chosen microwave pulses can increase the amplitude of coherent oscillations between cavity and spin ensemble by two orders of magnitude.
Gauge invariance is the cornerstone of modern quantum field theory. Recently, it has been shown that the quantum Rabi model, describing the dipolar coupling between a two-level atom and a quantized electromagnetic field, violates this principle. This widely used model describes a plethora of quantum systems and physical processes under different interaction regimes. In the ultrastrong coupling regime, it provides predictions which drastically depend on the chosen gauge. This failure is attributed to the finite-level truncation of the matter system. We show that a careful application of the gauge principle is able to restore gauge invariance even for extreme light-matter interaction regimes. The resulting quantum Rabi Hamiltonian in the Coulomb gauge differs significantly from the standard model and provides the same physical results obtained by using the dipole gauge. It contains field operators to all orders that cannot be neglected when the coupling strength is high. These results shed light on subtleties of gauge invariance in nonperturbative and extreme interaction regimes, which are now experimentally accessible, and solve all the long-lasting controversies arising from gauge ambiguities in the quantum Rabi and Dicke models.
The strong-coupling regime of cavity-quantum-electrodynamics (cQED) represents light-matter interaction at the fully quantum level. Adding a single photon shifts the resonance frequencies, a profound nonlinearity. cQED is a test-bed of quantum optics and the basis of photon-photon and atom-atom entangling gates. At microwave frequencies, success in cQED has had a transformative effect. At optical frequencies, the gates are potentially much faster and the photons can propagate over long distances and be easily detected, ideal features for quantum networks. Following pioneering work on single atoms, solid-state implementations are important for developing practicable quantum technology. Here, we embed a semiconductor quantum dot in a microcavity. The microcavity has a $mathcal{Q}$-factor close to $10^{6}$ and contains a charge-tunable quantum dot with close-to-transform-limited optical linewidth. The exciton-photon coupling rate $g$ exceeds both the photon decay rate $kappa$ and exciton decay rate $gamma$ by a large margin ($g/gamma=14$, $g/kappa=5.3$); the cooperativity is $C=2g^{2}/(gamma kappa)=150$, the $beta$-factor 99.7%. We observe pronounced vacuum Rabi oscillations in the time-domain, photon blockade at a one-photon resonance, and highly bunched photon statistics at a two-photon resonance. We use the change in photon statistics as a sensitive spectral probe of transitions between the first and second rungs of the Jaynes-Cummings ladder. All experiments can be described quantitatively with the Jaynes-Cummings model despite the complexity of the solid-state environment. We propose this system as a platform to develop optical-cQED for quantum technology, for instance a photon-photon entangling gate.