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All-optical reshaping of light pulses using $chi^{(2)}$ media

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 Added by Thomas Coudreau
 Publication date 2003
  fields Physics
and research's language is English




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We have developed a new method based on two cavities containing $chi^{(2)}$ media to reshape optical pulses by an all-optical technique. The system is entirely passive emph{i.e.}, all the energy is brought by the incoming pulse and uses two successive optical cavities with independent thresholds. The output pulse is close to a rectangular shape. We show that this technique could be extended to high bit rates and telecommunication wavelength using very small cavities containing current nonlinear materials.



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A two-level medium, described by the Maxwell-Bloch (MB) system, is engraved by establishing a standing cavity wave with a linearly polarized electromagnetic field that drives the medium on both ends. A light pulse, polarized along the other direction, then scatters the medium and couples to the cavity standing wave by means of the population inversion density variations. We demonstrate that control of the applied amplitudes of the grating field allows to stop the light pulse and to make it move backward (eventually to drive it freely). A simplified limit model of the MB system with variable boundary driving is obtained as a discrete nonlinear Schroedinger equation with tunable external potential. It reproduces qualitatively the dynamics of the driven light pulse.
Optical parametric oscillators (OPOs) have been widely used for decades as tunable, narrow linewidth, and coherent light sources for reaching long wavelengths and are attractive for applications such as quantum random number generation and Ising machines. To date, waveguide-based OPOs have suffered from relatively high thresholds on the order of hundreds of milliwatts. With the advance in integrated photonic techniques demonstrated by high-efficiency second harmonic generation in aluminum nitride (AlN) photonic microring resonators, highly compact and nanophotonic implementation of parametric oscillation is feasible. Here, we employ phase-matched AlN microring resonators to demonstrate low-threshold parametric oscillation in the telecom infrared band with an on-chip efficiency up to 17% and milliwatt-level output power. A broad phase-matching window is observed, enabling tunable generation of signal and idler pairs over a 180 nm bandwidth across the C band. This result establishes an important milestone in integrated nonlinear optics and paves the way towards chip-based quantum light sources and tunable, coherent radiation for spectroscopy and chemical sensing.
Mid-infrared laser frequency combs are compelling sources for precise and sensitive metrology with applications in molecular spectroscopy and spectro-imaging. The infrared atmospheric window between 3-5.5 $mu$m in particular provides vital information regarding molecular composition. Using a robust, fiber-optic source of few-cycle pulses in the near-infrared, we experimentally demonstrate ultra-broad bandwidth nonlinear phenomena including harmonic and difference frequency generation in a single pass through periodically poled lithium niobate (PPLN). These $chi^{(2)}$ nonlinear optical processes result in the generation of frequency combs across the mid-infrared atmospheric window which we employ for dual-comb spectroscopy of acetone and carbonyl sulfide with resolution as high as 0.003 cm$^{-1}$. Moreover, cascaded $chi^{(2)}$ nonlinearities in the same PPLN directly provide the carrier-envelope offset frequency of the near-infrared driving pulse train in a compact geometry.
Quadratic nonlinear processes are currently exploited for frequency comb transfer and extension from the visible and near infrared regions to other spectral ranges where direct comb generation cannot be accomplished. However, frequency comb generation has been directly observed in continuously-pumped quadratic nonlinear crystals placed inside an optical cavity. At the same time, an introductory theoretical description of the phenomenon has been provided, showing a remarkable analogy with the dynamics of third-order Kerr microresonators. Here, we give an overview of our recent work on $chi^{(2)}$ frequency comb generation. Furthermore, we generalize the preliminary three-wave spectral model to a many-mode comb and present a stability analysis of different cavity field regimes. Although at a very early stage, our work lays the groundwork for a novel class of highly efficient and versatile frequency comb synthesizers based on second-order nonlinear materials.
Optical frequency combs (OFCs) at Mid-Infrared (MIR) wavelengths are essential for applications in precise spectroscopy, gas sensing and molecular fingerprinting, because of its revolutionary precision in both wavelength and frequency domain. The microresonator-based OFCs make a further step towards practical applications by including such high precision in a compact and cost-effective package. However, dispersion engineering is still a challenge for the conventional chi-3 micro-ring resonators and a MIR pump laser is required. Here we develop a different platform of a chi-2 optical superlattice box resonator to generate MIR OFC by optical parametric down conversion. With near-material-limited quality factor of 2.0*10^7, broadband MIR OFC can be generated with over 250 nm span around 2060 nm, where only a common near-infrared laser is necessary as pump. The fine teeth spacing corresponds to a measurable radio frequency beat note at 1.566 GHz, and also results in a fine spectroscopy resolution. Its linewidth is measured to be 6.1 kHz, which reveals a low comb noise that agrees well with the clean temporal waveforms. With high output power of over 370 mW, such MIR OFC is capable for long distance sensing and ranging applications.
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