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Register a new userNon-Observation of the Production of Superheavy Nuclei in the Reaction of $^{86]$Kr with $^{208}$Pb
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Authors
K.E. Gregorich
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The published claim for the discovery of element 118 is retracted.
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In April-May, 2001, the previously reported experiment to synthesize element 118 using the $^{208}$Pb($^{86}$Kr,n)$^{293}$118 reaction was repeated. No events corresponding to the synthesis of element 118 were observed with a total beam dose of 2.6 x 10$^{18}$ ions. The simple upper limit cross sections (1 event) were 0.9 and 0.6 pb for evaporation residue magnetic rigidities of 2.00 $T m$ and 2.12 $T m$, respectively. A more detailed cross section calculation, accounting for an assumed narrow excitation function, the energy loss of the beam in traversing the target and the uncertainty in the magnetic rigidity of the Z=118 recoils is also presented. Re-analysis of the primary data files from the 1999 experiment showed the reported element 118 events are not in the original data. The current results put constraints on the production cross section for synthesis of very heavy nuclei in cold fusion reactions.
In the late stages of stellar core-collapse, prior to core bounce, electron captures on medium-heavy nuclei drive deleptonization and simulations require the use of accurate reaction rates. Nuclei with neutron number near $N=50$, just above atomic number $Z=28$, play an important role, but rates used in astrophysical simulations rely primarily on a relatively simple single-state approximation. In order to improve the accuracy of astrophysical simulations, experimental data are needed to test the electron-capture rates and to guide the development of better theoretical models. This work presents the results of the $^{86}$Kr($t$,$^{3}$He+$gamma$) experiment at the NSCL, from which an upper limit for the Gamow-Teller strength up to an excitation energy in $^{86}$Br of 5 MeV is extracted. The derived upper limit for the electron-capture rate on $^{86}$Kr indicates that the rate estimated through the single-state approximation is too high and that rates based on Gamow-Teller strengths estimated in shell-model and QRPA calculations are more accurate. The QRPA calculations tested in this manner were used for estimating the electron capture rates for 78 isotopes near $N=50$ and above $Z=28$. The impact of using these new electron-capture rates in simulations of supernovae instead of the rates based on the single-state approximation is investigated, indicating a significant reduction in the deleptonization that affects multi-messenger signals, such as the emission of neutrinos and gravitational waves.
The yields of over 200 projectile-like fragments (PLFs) and target-like fragments (TLFs) from the interaction of (E$_{c.m.}$=450 MeV) $^{136}$Xe with a thick target of $^{208}$Pb were measured using Gammasphere and off-line $gamma$-ray spectroscopy, giving a comprehensive picture of the production cross sections in this reaction.The measured yields were compared to predictions of the GRAZING model and the predictions of Zagrebaev and Greiner using a quantitative metric, the theory evaluation factor, {bf tef}. The GRAZING model predictions are adequate for describing the yields of nuclei near the target or projectile but grossly underestimate the yields of all other products. The predictions of Zagrebaev and Greiner correctly describe the magnitude and maxima of the observed TLF transfer cross sections for a wide range of transfers ($Delta$Z = -8 to $Delta$Z = +2). However for $Delta$Z =+4, the observed position of the maximum in the distribution is four neutrons richer than the predicted maximum. The predicted yields of the neutron-rich N=126 nuclei exceed the measured values by two orders of magnitude. Correlations between TLF and PLF yields are discussed.
We measured fragmentation cross sections produced using the primary beam of $^{86}$Kr at 64 MeV/nucleon on $^9$Be and $^{181}$Ta targets. The cross sections were obtained by integrating the momentum distributions of isotopes with 25<Z<36 measured using the RIPS fragment separator at RIKEN. The cross-section ratios obtained with the $^{181}$Ta and $^{9}$Be targets depend on the fragment masses, contrary to the simple geometrical models. We compared the extracted cross sections to EPAX; an empirical parameterization of fragmentation cross sections. Predictions from current EPAX parameterization severely overestimate the production cross sections of very neutron-rich isotopes. Attempts to obtain another set of EPAX parameters specific to the reaction studied here, to extrapolate the neutron-rich nuclei more accurately have not been very successful, suggesting that accurate predictions of production cross sections of nuclei far from the valley of stability require information of nuclear properties which are not present in EPAX.
The evolution of nuclear magic numbers at extremes of isospin is a topic at the forefront of contemporary nuclear physics. $N=50$ is a prime example, with increasing experimental data coming to light on potentially doubly-magic $^{100}$Sn and $^{78}$Ni at the proton-rich and proton-deficient extremes, respectively. Experimental discrepancies exist in the data for less exotic systems. In $^{86}$Kr the $B(E2;2^+_1rightarrow0^+_1)$ value - a key indicator of shell evolution - has been experimentally determined by two different methodologies, with the results deviating by $3sigma$. Here, we report on a new high-precision measurement of this value, as well as the first measured lifetimes and hence transition strengths for the $2^+_2$ and $3^-_{(2)}$ states in the nucleus. The Doppler-shift attenuation method was implemented using the TIGRESS gamma-ray spectrometer and TIGRESS integrated plunger (TIP) device. High-statistics Monte-Carlo simulations were utilized to extract lifetimes in accordance with state-of-the-art methodologies. Lifetimes of $tau(2^+_1)=336pm4text{(stat.)}pm20text{(sys.)}$ fs, $tau(2^+_2)=263pm9text{(stat.)}pm19text{(sys.)}$ fs and $tau(3^-_{(2)})=73pm6text{(stat.)}pm32text{(sys.)}$ fs were extracted. This yields a transition strength for the first-excited state of $B(E2;2^+_1rightarrow0^+)=259pm3text{(stat.)}pm16text{(sys.)}$ e$^2$fm$^4$. The measured lifetime disagrees with the previous Doppler-shift attenuation method measurement by more than $3sigma$, while agreeing well with a previous value extracted from Coulomb excitation. The newly extracted $B(E2;2^+_1rightarrow0^+_1)$ value indicates a more sudden reduction in collectivity in the $N=50$ isotones approaching $Z=40$.
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