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Using spin-density-functional theory, we study the electronic states of a two-dimensional parabolic quantum dot with up to N=58 electrons. We observe a shell structure for the filling of the dot with electrons. Hunds rule determines the spin configuration of the ground state, but only up to 22 electrons. At specific N, the ground state is degenerate, and a small elliptical deformation of the external potential induces a rotational charge-density-wave (CDW) state. Previously identified spin-density-wave (SDW) states are shown to be artifacts of broken spin symmetry in density-functional theory.
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Confined states of a positronium (Ps) in the spherical and circular quantum dots (QDs) are theoretically investigated in two size-quantization regimes: strong and weak. Two-band approximation of Kane dispersion law and parabolic dispersion law of charge carriers are considered. It is shown that the electronpositron pair instability is a consequence of dimensionality reduction, not of the size quantization (SQ). The binding energies for the Ps in circular and spherical QDs are calculated. The Ps formation dependence on the QD radius is studied.
We study ground states and excited states in semiconductor quantum dots containing 1 to 12 electrons. For the first time, it is possible to identify the quantum numbers of the states in the excitation spectra and make a direct comparison to exact calculations. A magnetic field induces transitions between excited states and ground state. These transitions are discussed in terms of crossings between single-particle states, singlet-triplet transitions, spin polarization, and Hunds rule. Our impurity-free quantum dots allow for atomic physics experiments in magnetic field regimes not accessible for atoms.
We have investigated the magnetoplasmon excitations in arrays of circular and noncircular quantum dots within the Thomas-Fermi-Dirac-von Weizsacker approximation. Deviations from the ideal collective excitations of isolated parabolically confined electrons arise from local perturbations of the confining potential as well as interdot Coulomb interactions. The latter are unimportant unless the interdot separations are of the order of the size of the dots. Local perturbations such as radial anharmonicity and noncircular symmetry lead to clear signatures of the violation of the generalized Kohn theorem. In particular, the reduction of the local symmetry from SO(2) to $C_4$ results in a resonant coupling of different modes and an observable anticrossing behaviour in the power absorption spectrum. Our results are in good agreement with recent far-infrared (FIR) transmission experiments.
The authors report that anisotropic confining potentials in laterally-coupled semiconductor quantum dots (QDs) have large impacts in optical transitions and energies of inter-shell collective electronic excitations. The observed anisotropies are revealed by inelastic light scattering as a function of the in-plane direction of light polarization and can be finely controlled by modifying the geometrical shape of the QDs. These experiments show that the tuning of the QD confinement potential offers a powerful method to manipulate electronic states and far-infrared inter-shell optical transitions in quantum dots.
We theoretically investigate the properties of holes in a Si$_{x}$Ge$_{1-x}$/Ge/ Si$_{x}$Ge$_{1-x}$ quantum well in a perpendicular magnetic field that make them advantageous as qubits, including a large ($>$100~meV) intrinsic splitting between the light and heavy hole bands, a very light ($sim$0.05$, m_0$) in-plane effective mass, consistent with higher mobilities and tunnel rates, and larger dot sizes that could ameliorate constraints on device fabrication. Compared to electrons in quantum dots, hole qubits do not suffer from the presence of nearby quantum levels (e.g., valley states) that can compete with spins as qubits. The strong spin-orbit coupling in Ge quantum wells may be harnessed to implement electric-dipole spin resonance, leading to gate times of several nanoseconds for single-qubit rotations. The microscopic mechanism of this spin-orbit coupling is discussed, along with its implications for quantum gates based on electric-dipole spin resonance, stressing the importance of coupling terms that arise from the underlying cubic crystal field. Our results provide a theoretical foundation for recent experimental advances in Ge hole-spin qubits.
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