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Register a new userState Selection in Accelerated Systems
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Authors
Martin Tarlie
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The problem of state selection when multiple metastable states compete for occupation is considered for systems that are accelerated far from equilibrium. The dynamics of the supercurrent in a narrow superconducting ring under the influence of an external electric field is used to illustrate the general phenomenology.
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The kagome Heisenberg antiferromagnet is a leading candidate in the search for a spin system with a quantum spin-liquid ground state. The nature of its ground state remains a matter of great debate. We conducted 17-O single crystal NMR measurements of the S=1/2 kagome lattice in herbertsmithite ZnCu$_3$(OH)$_6$Cl$_2$, which is known to exhibit a spinon continuum in the spin excitation spectrum. We demonstrate that the intrinsic local spin susceptibility $chi_{kagome}$ deduced from the 17-O NMR frequency shift asymptotes to zero below temperature T ~ 0.03 J, where J ~ 200 K is the Cu-Cu super-exchange interaction. Combined with the magnetic field dependence of $chi_{kagome}$ we observed at low temperatures, these results imply that the kagome Heisenberg antiferromagnet has a spin-liquid ground state with a finite gap.
We study the statistical mechanics of counterion Wigner crystals associated with hexagonal bundles of chiral biopolymers. We show that, due to spontaneous chiral symmetry breaking induced by frustration, these Wigner crystals would be chiral even if the biopolymers themselves were not chiral. Using a duality transformation of the model onto a spin-charge Hamiltonian, we show that melting of the Wigner crystal is due to the unbinding of screw dislocations and that the melting temperature has a singular dependence on the intrinsic chirality of the biopolymers. Finally, we report that, if electrostatic interactions are strongly screened, the counterions can condense in the form of an intermediate achiral Wigner solid phase that melts by the unbinding of fractional topological charges.
The net charge of solvated entities, ranging from polyelectrolytes and biomolecules to charged nanoparticles and membranes, depends on the local dissociation equilibrium of individual ionizable groups. Incorporation of this phenomenon, emph{charge regulation}, in theoretical and computational models requires dynamic, configuration-dependent recalculation of surface charges and is therefore typically approximated by assuming constant net charge on particles. Various computational methods exist that address this. We present an alternative, particularly efficient charge regulation Monte Carlo method (CR-MC), which explicitly models the redistribution of individual charges and accurately samples the correct grand-canonical charge distribution. In addition, we provide an open-source implementation in the LAMMPS molecular dynamics (MD) simulation package, resulting in a hybrid MD/CR-MC simulation method. This implementation is designed to handle a wide range of implicit-solvent systems that model discreet ionizable groups or surface sites. The computational cost of the method scales linearly with the number of ionizable groups, thereby allowing accurate simulations of systems containing thousands of individual ionizable sites. By matter of illustration, we use the CR-MC method to quantify the effects of charge regulation on the nature of the polyelectrolyte coil--globule transition and on the effective interaction between oppositely charged nanoparticles.
We propose a fully operational framework to study the non-equilibrium thermodynamics of a quantum system $S$ that is coupled to a detector $D$ whose state is continuously monitored, allowing to single out individual quantum trajectories of $S$. We focus on detailed fluctuation theorems and characterize the entropy production of the system. We establish fundamental differences with respect to the thermodynamic of unmonitored, unitarily evolved systems. We consider the paradigmatic example of circuit-QED, where superconducting qubits can be coupled to a continuously monitored resonator and show numerical simulations using state of the art experimental parameters.
We consider a single down atom within a Fermi sea of up atoms. We elucidate by a full many-body analysis the quite mysterious agreement between Monte-Carlo results and approximate calculations taking only into account single particle-hole excitations. It results from a nearly perfect destructive interference of the contributions of states with more than one particle-hole pair. This is linked to the remarkable efficiency of the expansion in powers of hole wavevectors, the lowest order leading to perfect interference. Going up to two particle-hole pairs gives an essentially perfect agreement with known exact results. Hence our treatment amounts to an exact solution of this problem.
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