No Arabic abstract
We develop a theory of magnetoresistance based on variable-range hopping. An exponentially large, low-field and necessarily positive magnetoresistance effect is predicted in the presence of Hubbard interaction and spin-dynamics under certain conditions. The theory was developed with the recently discovered organic magnetoresistance in mind. To account for the experimental observation that the organic magnetoresistance effect can also be negative, we tentatively amend the theory with a mechanism of bipolaron formation.
We predict the universal power law dependence of localization length on magnetic field in the strongly localized regime. This effect is due to the orbital quantum interference. Physically, this dependence shows up in an anomalously large negative magnetoresistance in the hopping regime. The reason for the universality is that the problem of the electron tunneling in a random media belongs to the same universality class as directed polymer problem even in the case of wave functions of random sign. We present numerical simulations which prove this conjecture. We discuss the existing experiments that show anomalously large magnetoresistance. We also discuss the role of localized spins in real materials and the spin polarizing effect of magnetic field.
Using molecular dynamics simulations we study the static and dynamic properties of spherical nanoparticles (NPs) embedded in a disordered and polydisperse polymer network. Purely repulsive (RNP) as well as weakly attractive (ANP) polymer-NP interactions are considered. It is found that for both types of particles the NP dynamics at intermediate and at long times is controlled by the confinement parameter $C=sigma_N/lambda$, where $sigma_N$ is the NP diameter and $lambda$ is the dynamic localization length of the crosslinks. Three dynamical regimes are identified: i) For weak confinement ($C lesssim 1$) the NPs can freely diffuse through the mesh; ii) For strong confinement ($C gtrsim 1$) NPs proceed by means of activated hopping; iii) For extreme confinement ($C gtrsim 3$) the mean squared displacement shows on intermediate time scales a quasi-plateau since the NPs are trapped by the mesh for very long times. Escaping from this local cage is a process that depends strongly on the local environment, thus giving rise to an extremely heterogeneous relaxation dynamics. The simulation data are compared with the two main theories for the diffusion process of NPs in gels. Both theories give a very good description of the $C-$dependence of the NP diffusion constant, but fail to reproduce the heterogeneous dynamics at intermediate time scales.
Anomalous Hall effect (AHE) is important for understanding the topological properties of electronic states, and provides insight into the spin-polarized carriers of magnetic materials. AHE has been extensively studied in metallic, but not variable-range-hopping (VRH), regime. Here we report the experiments of both anomalous and ordinary Hall effect (OHE) in Mott and Efros VRH regimes. We found unusual scaling law of the AHE coefficient $Rah=aRxx^b$ with b>2, contrasting the OHE coefficient $Roh=cRxx^d$ with d<1. More strikingly, the sign of AHE coefficient changes with temperature with specific electron densities.
We study spin transport in a Hubbard chain with strong, random, on--site potential and with spin--dependent hopping integrals, $t_{sigma}$. For the the SU(2) symmetric case, $t_{uparrow} =t_{downarrow}$, such model exhibits only partial many-body localization with localized charge and (delocalized) subdiffusive spin excitations. Here, we demonstrate that breaking the SU(2) symmetry by even weak spin--asymmetry, $t_{uparrow} e t_{downarrow}$, localizes spins and restores full many-body localization. To this end we derive an effective spin model, where the spin subdiffusion is shown to be destroyed by arbitrarily weak $t_{uparrow} e t_{downarrow}$. Instability of the spin subdiffusion originates from an interplay between random effective fields and singularly distributed random exchange interactions.
We generalize the force-level, microscopic, Nonlinear Langevin Equation (NLE) theory and its elastically collective generalization (ECNLE theory) of activated dynamics in bulk spherical particle liquids to address the influence of random particle pinning on structural relaxation. The simplest neutral confinement model is analyzed for hard spheres where there is no change of the equilibrium pair structure upon particle pinning. As the pinned fraction grows, cage scale dynamical constraints are intensified in a manner that increases with density. This results in the mobile particles becoming more transiently localized, with increases of the jump distance, cage scale barrier and NLE theory mean hopping time; subtle changes of the dynamic shear modulus are predicted. The results are contrasted with recent simulations. Similarities in relaxation behavior are identified in the dynamic precursor regime, including a roughly exponential, or weakly supra-exponential, growth of the alpha time with pinning fraction and a reduction of dynamic fragility. However, the increase of the alpha time with pinning predicted by the local NLE theory is too small, and severely so at very high volume fractions. The strong deviations are argued to be due to the longer range collective elasticity aspect of the problem which is expected to be modified by random pinning in a complex manner. A qualitative physical scenario is offered for how the three distinct aspects that quantify the elastic barrier may change with pinning. ECNLE theory calculations of the alpha time are then presented based on the simplest effective-medium-like treatment for how random pinning modifies the elastic barrier. The results appear to be consistent with most, but not all, trends seen in recent simulations. Key open problems are discussed with regards to both theory and simulation.