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Erratum: Dynamics and scaling in a quantum spin chain material with bond randomness

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 Added by Andrey Zheludev
 Publication date 2004
  fields Physics
and research's language is English




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Follow-up neutron measurements, performed on a sample much larger than the one used in the original study, show that in the energy range 0.5-45 meV the magnetic excitations in BaCu2SiGeO7 are indistinguishable from those in conventional (disorder-free) quantum S=1/2 chains. Scrutinizing the previous data, we found that the analysis was affected by a poorly identified structured background and an additional technical mistake in the data reduction.



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We carried out AC magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ~1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type ground state, i.e. without broken symmetries or frozen moments. However, the AC susceptibility revealed a dilute-spin-glass like transition below ~ 1 K. Antiferromagnetically coupled Mo5+ 4d1 electrons in triply degenerate t2g orbitals are in this material arranged in a geometrically frustrated fcc lattice. Bulk magnetic susceptibility data has previously been interpreted in terms of a freezing to a heterogeneous state with non-magnetic sites where 4d^1 electrons have paired in spin-singlets dimers, and residual unpaired Mo5+ 4d1 electrons. Based on the magnetic heat capacity data it has been suggested that this heterogeneity is the result of kinetic constraints intrinsic to the physics of the pure system (possibly due to topological overprotection), leading to a self-induced glass of valence bonds between neighbouring 4d1 electrons. The muSR relaxation unambiguously points to a static heterogeneous state with a static arrangement of unpaired electrons isolated by spin-singlet (valence bond) dimers between the majority of Mo5+ 4d electrons. The AC susceptibility data indicate that the residual magnetic moments freeze into a dilute-spin-glass-like state. This is in apparent contradiction with the muon-spin decoupling at 50 mK in fields up to 200 mT, which indicates that, remarkably, the time scale of the field fluctuations from the residual moments is ~ 5 ns. Comparable behaviour has been observed in other geometrically frustrated magnets with spin-liquid-like behaviour and the implications of our observations on Ba2YMoO6 are discussed in this context.
We study spin transport in a Hubbard chain with strong, random, on--site potential and with spin--dependent hopping integrals, $t_{sigma}$. For the the SU(2) symmetric case, $t_{uparrow} =t_{downarrow}$, such model exhibits only partial many-body localization with localized charge and (delocalized) subdiffusive spin excitations. Here, we demonstrate that breaking the SU(2) symmetry by even weak spin--asymmetry, $t_{uparrow} e t_{downarrow}$, localizes spins and restores full many-body localization. To this end we derive an effective spin model, where the spin subdiffusion is shown to be destroyed by arbitrarily weak $t_{uparrow} e t_{downarrow}$. Instability of the spin subdiffusion originates from an interplay between random effective fields and singularly distributed random exchange interactions.
We investigate and contrast, via entropic sampling based on the Wang-Landau algorithm, the effects of quenched bond randomness on the critical behavior of two Ising spin models in 2D. The random bond version of the superantiferromagnetic (SAF) square model with nearest- and next-nearest-neighbor competing interactions and the corresponding version of the simple Ising model are studied and their general universality aspects are inspected by a detailed finite-size scaling (FSS) analysis. We find that, the random bond SAF model obeys weak universality, hyperscaling, and exhibits a strong saturating behavior of the specific heat due to the competing nature of interactions. On the other hand, for the random Ising model we encounter some difficulties for a definite discrimination between the two well-known scenarios of the logarithmic corrections versus the weak universality. Yet, a careful FSS analysis of our data favors the field-theoretically predicted logarithmic corrections.
Quantum nematic phases are analogous to classical liquid crystals. Like liquid crystals, which break the rotational symmetries of space, their quantum analogues break the point-group symmetry of the crystal due to strong electron-electron interactions, as in quantum Hall states, Sr3Ru2O7, and high temperature superconductors. Here, we present angle resolved magnetoresistance (AMRO) measurements that reveal a quantum nematic phase in the hexaboride EuB6. We identify the region in the temperature-magnetic field phase diagram where the magnetoresistance shows two-fold oscillations instead of the expected four-fold pattern. This is the same region where magnetic polarons were previously observed, suggesting that they drive the nematicity in EuB6. This is also the region of the phase diagram where EuB6 shows a colossal magnetoresistance (CMR). This novel interplay between magnetic and electronic properties could thus be harnessed for spintronic applications.
The rounding of first order phase transitions by quenched randomness is stated in a form which is applicable to both classical and quantum systems: The free energy, as well as the ground state energy, of a spin system on a $d$-dimensional lattice is continuously differentiable with respect to any parameter in the Hamiltonian to which some randomness has been added when $d leq 2$. This implies absence of jumps in the associated order parameter, e.g., the magnetization in case of a random magnetic field. A similar result applies in cases of continuous symmetry breaking for $d leq 4$. Some questions concerning the behavior of related order parameters in such random systems are discussed.
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