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Register a new userMagnons in CMR pyrochlore Tl2Mn2O7
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Well defined spin waves were observed when the spin dynamics of Tl2Mn2O7, the first pyrochlore compound found to exhibit colossal magnetoresistance, was measured [J.W.Lynn et al., Phys.Rev.Lett. 80,4582(1998)], in stark contrast with the experimental results on the larger family of magnetoresistive manganites with perovskite structure. In this work, we present our calculation for the spin waves in Tl2Mn2O7, which we described using the microscopic generic model proposed recently for this compound [C.I.Ventura and M.A.Gusmao, Phys.Rev.B 65, 14422(2002)]. We have employed a canonical transformation to determine perturbatively the effective spin-wave Hamiltonian, obtaining therefrom the renormalization of the ferromagnetic spin waves related to the localized Mn$^{4+}$ spins, due to their coupling with the conduction electrons present. We have calculated the magnon dispersion relations along different paths in the first Brillouin zone, comparing them with those which are obtained for an ideal isotropic ferromagnet. This comparison evidences an agreement between the ferromagnetic magnons obtained from the generic model and the bare spin waves, such as had been found in neutron scattering experiments.
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We report the low temperature magnetic properties of Nd$^{3+}$ pyrochlore $rm Nd_2ScNbO_7$. Susceptibility and magnetization show an easy-axis moment, and heat capacity reveals a phase transition to long range order at $T_N=371(2)$ mK with a fully recovered $Delta S = R ln(2)$, 53% of it recovered for $T>T_N$. Elastic neutron scattering shows a long-range all-in-all-out magnetic order with low-$Q$ diffuse elastic scattering. Inelastic neutron scattering shows a low-energy flat-band, indicating a magnetic Hamiltonian similar to $rm Nd_2Zr_2O_7$. Nuclear hyperfine excitations measured by ultra-high-resolution neutron backscattering indicates a distribution of static electronic moments below $T_N$, which may be due to B-site disorder influencing Nd crystal electric fields. Analysis of heat capacity data shows an unexpected $T$-linear or $T^{3/2}$ term which is inconsistent with conventional magnon quasiparticles, but is consistent with fractionalized spinons or gapless local spin excitations. We use legacy data to show similar behavior in $rm Nd_2Zr_2O_7$. Comparing local static moments also reveals a suppression of the nuclear Schottky anomaly in temperature, evidencing a fraction of Nd sites with nearly zero static moment, consistent with exchange-disorder-induced random singlet formation. Taken together, these measurements suggest an unusual fluctuating magnetic ground state which mimics a spin-liquid -- but may not actually be one.
We report on resistivity measurements in La$_{0.67}$Ca$_{0.33}$MnO$_{3}$ and Nd$_{0.7}$Sr$_{0.3}$MnO$_{3}$ thin films in order to elucidate the underlying mechanism for the CMR behavior. The experimental results are analyzed in terms of quantum phase transition ideas to study the nature of the metal-insulator transition in manganese oxides. Resistivity curves as functions of magnetization for various temperatures show the absence of scaling behavior expected in a continuous quantum phase transition, which leads us to conclude that the observed metal-insulator transition is most likely a finite temperature crossover phenomenon.
We analyze the magnon excitations in pyrochlore iridates with all-in-all-out (AIAO) antiferromagnetic order, focusing on their topological features. We identify the magnetic point group symmetries that protect the nodal-line band crossings and triple-point degeneracies that dominate the Berry curvature. We find three distinct regimes of magnon band topology, as a function of the ratio of Dzyaloshinskii-Moriya (DM) interaction to the antiferromagnetic exchange. We show how the thermal Hall response provides a unique probe of the topological magnon band structure in AIAO systems.
We investigate the low-temperature electron, lattice, and spin dynamics of LaMnO_3 (LMO) and La_0.7Ca_0.3MnO_3 (LCMO) by resonant pump-probe reflectance spectroscopy. Probing the high-spin d-d transition as a function of time delay and probe energy, we compare the responses of the Mott insulator and the double-exchange metal to the photoexcitation. Attempts have previously been made to describe the sub-picosecond dynamics of CMR manganites in terms of a phenomenological three temperature model describing the energy transfer between the electron, lattice and spin subsystems followed by a comparatively slow exponential decay back to the ground state. However, conflicting results have been reported. Here we first show clear evidence of an additional component in the long term relaxation due to film-to-substrate heat diffusion and then develop a modified three temperature model that gives a consistent account for this feature. We confirm our interpretation by using it to deduce the bandgap in LMO. In addition we also model the non-thermal sub-picosecond dynamics, giving a full account of all observed transient features both in the insulating LMO and the metallic LCMO.
We investigated the temperature-dependent optical conductivity of NaV2O5 in the energy range 4 meV-4 eV. The intensities and the polarization dependence of the detected electronic excitations give a direct indication for a broken-parity electronic ground-state and for a non-centrosymmetric crystal structure of the system in the high-temperature phase. A direct two-magnon optical absorption process, proposed in this Letter, is in quantitative agreement with the optical data. By analyzing the optically allowed phonons at various temperatures above and below the phase transition, we conclude that a second-order change to a larger unit cell takes place below 34 K.
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