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Register a new userSpecific Heat of CeRhIn5: Pressure-Driven Evolution of the Ground State from Antiferromagnetism to Superconductivity
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Measurements of the specific heat of antiferromagnetic CeRhIn5, to 21 kbar, and for 21 kbar to 70 kOe, show a discontinuous change from an antiferromagnetic ground state below 15 kbar to a superconducting ground state above, and suggest that it is accompanied by a weak thermodynamic first-order transition. Bulk superconductivity appears, apparently with d-wave electron pairing, at the critical pressure, 15 kbar; with further increase in pressure a residual temperature-proportional term in the specific heat disappears.
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We report on detailed ac calorimetry measurements under high pressure and magnetic field of CeRhIn5. Under hydrostatic pressure the antiferromagnetic order vanishes near p_c*=2 GPa due to a first order transition. Superconductivity is found for pressures above 1.5 GPa inside the magnetic ordered phase. However, the superconductivity differ from the pure homogeneous superconducting ground state above 2 GPa. The application of an external magnetic field H || ab induces a transition inside the superconducting state above pc* which is strongly related to the re-entrance of the antiferromagnetism with field. This field-induced supplementary state vanishes above the quantum critical point in this system. The analogy to CeCoIn5 is discussed.
The effect of substituting Rh in CeRh1-xPdxIn5 with Pd up to x = 0.25 has been studied on single crystals. The crystals have been grown by means of the In self-flux method and characterized by x-ray diffraction and microprobe. The tetragonal HoCoGa5-type of structure and the c/a ratio of the parent compound remains intact by the Pd substitution; the unit cell volume increases by 0.6 % with x = 0.25 of Pd. The low-temperature behavior of resistivity was studied also under hydrostatic pressure up to 2.25 GPa. The Pd substitution for Rh affects the magnetic behavior and the maximum value of the superconducting transition temperature measured at pressures above 2 GPa only negligibly. On the other hand, the results provide evidence that superconductivity in CeRh0.75Pd0.25In5 is induced at significantly lower pressures, i.e. the Pd substitution for Rh shifts the CeRh1-xPdxIn5 system closer to coexistence of magnetism and superconductivity at ambient pressure.
The electronic ground state in many iridate materials is described by a complex wave-function in which spin and orbital angular momenta are entangled due to relativistic spin-orbit coupling (SOC). Such a localized electronic state carries an effective total angular momentum of $J_{eff}=1/2$. In materials with an edge-sharing octahedral crystal structure, such as the honeycomb iridates Li2IrO3 and Na2IrO3, these $J_{eff}=1/2$ moments are expected to be coupled through a special bond-dependent magnetic interaction, which is a necessary condition for the realization of a Kitaev quantum spin liquid. However, this relativistic electron picture is challenged by an alternate description, in which itinerant electrons are confined to a benzene-like hexagon, keeping the system insulating despite the delocalized nature of the electrons. In this quasi-molecular orbital (QMO) picture, the honeycomb iridates are an unlikely choice for a Kitaev spin liquid. Here we show that the honeycomb iridate Li2IrO3 is best described by a $J_{eff}=1/2$ state at ambient pressure, but crosses over into a QMO state under the application of small (~ 0.1 GPa) hydrostatic pressure. This result illustrates that the physics of iridates is extremely rich due to a delicate balance between electronic bandwidth, spin-orbit coupling, crystal field, and electron correlation.
We report $^{115}$In nuclear-quadrupole-resonance (NQR) measurements of the pressure($P$)-induced superconductor CeRhIn$_5$ in the antiferromagnetic (AF) and superconducting (SC) states. In the AF region, the internal field $H_{int}$ at the In site is substantially reduced from $H_{int}=1.75$ kOe at P=0 to 0.39 kOe at $P=1.23$ GPa, while the Neel temperature slightly changes with increasing $P$. This suggests that either the size in the ordered moment $M_{Q}(P)$ or the angle $theta (P)$ between the direction of $M_{Q}(P)$ and the tetragonal $c$ axis is extrapolated to zero at $P^*=1.6 pm 0.1$ GPa at which a bulk SC transition is no longer emergent. In the SC state at $P=2.1$ GPa, the nuclear spin-lattice relaxation rate $^{115}(1/T_1)$ has revealed a $T^3$ dependence without the coherence peak just below $T_c$, giving evidence for the unconventional superconductivity. The dimensionality of the magnetic flutuations in the normal state are also discussed.
Pressure-induced variations of $^{27}$Al NMR spectra of CeAl$_3$ indicate significant changes in the ground-state characteristics of this prototypical heavy-electron compound. Previously reported magnetic and electronic inhomogeneities at ambient pressure and very low temperatures are removed with external pressures exceeding 1.2 kbar. The spectra and results of corresponding measurements of the NMR spin-lattice relaxation rates indicate a pressure-induced emergence of a simple paramagnetic state involving electrons with moderately enhanced masses and no magnetic order above 65 mK.
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